Efficient and mechanically robust stretchable organic light-emitting devices by a laser-programmable buckling process

Stretchable organic light-emitting devices are becoming increasingly important in the fast-growing fields of wearable displays, biomedical devices and health-monitoring technology. Although highly stretchable devices have been demonstrated, their luminous efficiency and mechanical stability remain impractical for the purposes of real-life applications. This is due to significant challenges arising from the high strain-induced limitations on the structure design of the device, the materials used and the difficulty of controlling the stretch-release process. Here we have developed a laser-programmable buckling process to overcome these obstacles and realize a highly stretchable organic light-emitting diode with unprecedented efficiency and mechanical robustness. The strained device luminous efficiency −70 cd A −1 under 70% strain - is the largest to date and the device can accommodate 100% strain while exhibiting only small fluctuations in performance over 15,000 stretch-release cycles. This work paves the way towards fully stretchable organic light-emitting diodes that can be used in wearable electronic devices. Highly stretchable organic light-emitting diodes tend to suffer from a lack of mechanical robustness. Here, Yin et al . fabricate ordered buckled films by laying flexible light-emitting diodes on laser-ablated, prestretched substrates. The devices exhibit good emission stability over 15,000 stretching cycles.