Spiral spin liquid behavior and persistent reciprocal kagome structure in frustrated van der Waals magnets and beyond
We study classical J_{1}-J_{2} models with distinct spin degrees of freedom on a honeycomb lattice. For the XY and Heisenberg spins, the system develops a spiral spin liquid (SSL) that is a thermal cooperative paramagnetic regime with spins fluctuating around the spiral contours in the momentum spac...
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Veröffentlicht in: | Physical review research 2022-02, Vol.4 (1), p.013121, Article 013121 |
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Hauptverfasser: | , , |
Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | We study classical J_{1}-J_{2} models with distinct spin degrees of freedom on a honeycomb lattice. For the XY and Heisenberg spins, the system develops a spiral spin liquid (SSL) that is a thermal cooperative paramagnetic regime with spins fluctuating around the spiral contours in the momentum space, and at low temperatures supports a vector spin-chirality order despite the absence of long-range magnetic order. In a strong contrast, for the Ising moments, the low-temperature spin correlation forms a reciprocal kagome structure in the momentum space that resembles the SSL behaviors and persists for a range of exchange couplings. The unexpected emergence and persistence of the reciprocal kagome structure are attributed to the stiffness of the Ising moments and the frustration. At higher temperatures when the thermal fluctuations are strong and the spin correlation is not fully melted, the reciprocal structures evolve from kagome structure towards the ones demanded by the soft-spin limit. This contrasts strongly with the behaviors of the spiral contours in the SSL regime for the continuous spins. We suggest various experimentally relevant systems including van der Waals magnets such as the transition-metal phosphorus trichalcogenides TMPX_{3}, Cr_{2}Ge_{2}Te_{6}, the rare-earth chalcohalides (such as HoOF, ErOF, and DyOF), and other isostructural systems to realize the SSL-like behaviors and/or the reciprocal kagome structure. |
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ISSN: | 2643-1564 2643-1564 |
DOI: | 10.1103/PhysRevResearch.4.013121 |