10-year satellite-constrained fluxes of ammonia improve performance of chemistry transport models

In recent years, ammonia emissions have been continuously increasing, being almost 4 times higher than in the 20th century. Although an important species, as its use as a fertilizer sustains human living, ammonia has major consequences for both humans and the environment because of its reactive gas-...

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Veröffentlicht in:Atmospheric chemistry and physics 2021-03, Vol.21 (6), p.4431-4451
Hauptverfasser: Evangeliou, Nikolaos, Balkanski, Yves, Eckhardt, Sabine, Cozic, Anne, Van Damme, Martin, Coheur, Pierre-François, Clarisse, Lieven, Shephard, Mark W, Cady-Pereira, Karen E, Hauglustaine, Didier
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Sprache:eng
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Zusammenfassung:In recent years, ammonia emissions have been continuously increasing, being almost 4 times higher than in the 20th century. Although an important species, as its use as a fertilizer sustains human living, ammonia has major consequences for both humans and the environment because of its reactive gas-phase chemistry that makes it easily convertible to particles. Despite its pronounced importance, ammonia emissions are highly uncertain in most emission inventories. However, the great development of satellite remote sensing nowadays provides the opportunity for more targeted research on constraining ammonia emissions. Here, we used satellite measurements to calculate global ammonia emissions over the period 2008-2017. Then, the calculated ammonia emissions were fed to a chemistry transport model, and ammonia concentrations were simulated for the period 2008-2017.
ISSN:1680-7324
1680-7316
1680-7324
DOI:10.5194/acp-21-4431-2021