Two-dimensional heavy fermion in a monoatomic-layer Kondo lattice YbCu2

The Kondo effect between localized f -electrons and conductive carriers leads to exotic physical phenomena. Among them, heavy-fermion (HF) systems, in which massive effective carriers appear due to the Kondo effect, have fascinated many researchers. Dimensionality is also an important characteristic...

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Veröffentlicht in:Nature communications 2023-12, Vol.14 (1), p.7850-7850, Article 7850
Hauptverfasser: Nakamura, Takuto, Sugihara, Hiroki, Chen, Yitong, Yukawa, Ryu, Ohtsubo, Yoshiyuki, Tanaka, Kiyohisa, Kitamura, Miho, Kumigashira, Hiroshi, Kimura, Shin-ichi
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Sprache:eng
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Zusammenfassung:The Kondo effect between localized f -electrons and conductive carriers leads to exotic physical phenomena. Among them, heavy-fermion (HF) systems, in which massive effective carriers appear due to the Kondo effect, have fascinated many researchers. Dimensionality is also an important characteristic of the HF system, especially because it is strongly related to quantum criticality. However, the realization of the perfect two-dimensional (2D) HF materials is still a challenging topic. Here, we report the surface electronic structure of the monoatomic-layer Kondo lattice YbCu 2 on a Cu(111) surface observed by synchrotron-based angle-resolved photoemission spectroscopy. The 2D conducting band and the Yb 4 f state, located very close to the Fermi level, are observed. These bands are hybridized at low-temperature, forming the 2D HF state, with an evaluated coherence temperature of about 30 K. The effective mass of the 2D state is enhanced by a factor of 100 by the development of the HF state. Furthermore, clear evidence of the hybridization gap formation in the temperature dependence of the Kondo-resonance peak has been observed below the coherence temperature. Our study provides a new candidate as an ideal 2D HF material for understanding the Kondo effect at low dimensions. Examples of 2D heavy-fermion materials are rare, and the details of their electronic structure have remained elusive. Here, Nakamura et al. report the synthesis and angle-resolved photoemission spectroscopy measurements of a monolayer Kondo lattice, YbCu 2 , on a Cu(111) surface with an estimated coherence temperature of 30 K.
ISSN:2041-1723
2041-1723
DOI:10.1038/s41467-023-43662-9