Synthesis, characterization and up-conversion luminescence properties of alpha-NaYF4:Yb3+/Er3+/PVP/MOFs multilayer nanocrystals

The precursor PVP-capped α-NaYF4:Yb3+/Er3+ nanospheres were used as the templates for preparing the α-NaYF4:Yb3+/Er3+/PVP/MOFs multilayer nanocrystals with a self-template method. By using iron (III) carboxylate and zeolitic imidazolate frameworks dissolved in dimethylformamide (DMF) solution contai...

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Veröffentlicht in:Vietnam Journal of Science, Technology and Engineering Technology and Engineering, 2017-09, Vol.59 (3), p.79-84
Hauptverfasser: Lam, Thi Kieu Giang, Marciniak, Lukasz, Tran, Quang Huy, Dinh, Manh Tien, Vu, Duc Chinh, Nguyen, Vu, Tran, Thu Huong, Hoang, Thi Khuyen, Nguyen, Thanh Huong, Pham, Duc Roan, Nguyen, Thanh Binh, Le, Quoc Minh
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Sprache:eng
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Zusammenfassung:The precursor PVP-capped α-NaYF4:Yb3+/Er3+ nanospheres were used as the templates for preparing the α-NaYF4:Yb3+/Er3+/PVP/MOFs multilayer nanocrystals with a self-template method. By using iron (III) carboxylate and zeolitic imidazolate frameworks dissolved in dimethylformamide (DMF) solution containing 25% of diethylene glycol (DEG), the spherical-shaped α-NaYF4:Yb3+/Er3+/PVP/MIL-100 and α-NaYF4:Yb3+/Er3+/PVP/ZIF-8 multilayer nanocrystals were successfully prepared with the sizes of 300-500 nm at 100oC for one hour. Under a 976 nm laser excitation at room temperature, the α-NaYF4:Yb3+/Er3+/PVP/MIL-100 and α-NaYF4:Yb3+/Er3+/PVP/ZIF-8 multilayer nanocrystals exhibited strong up-conversion luminescence with three emission bands centered at around 520 nm, 540 nm, and 655 nm corresponding to 2H11/2 → 4I15/2, 4S3/2 → 4I15/2, and 4F9/2 → 4I15/2transitions of Er3+ ions, respectively.
ISSN:2525-2461
2615-9937
DOI:10.31276/VJSTE.59(3).79