Superfluidity of metastable glassy bulk para -hydrogen at low temperature

Molecular para-hydrogen (p-H sub(2)) has been proposed theoretically as a possible candidate for superfluidity, but the eventual superfluid transition is hindered by its crystallization. In this work, we study a metastable noncrystalline phase of bulk p-H sub(2) by means of the path integral Monte C...

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Veröffentlicht in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2012-06, Vol.85 (22), Article 224513
Hauptverfasser: Osychenko, O. N., Rota, R., Boronat, J.
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Sprache:eng
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Zusammenfassung:Molecular para-hydrogen (p-H sub(2)) has been proposed theoretically as a possible candidate for superfluidity, but the eventual superfluid transition is hindered by its crystallization. In this work, we study a metastable noncrystalline phase of bulk p-H sub(2) by means of the path integral Monte Carlo method in order to investigate at which temperature this system can support superfluidity. By choosing accurately the initial configuration and using a noncommensurate simulation box, we have been able to frustrate the formation of the crystal in the simulated system and to calculate the temperature dependence of the one-body density matrix and of the superfluid fraction. We observe a transition to a superfluid phase at temperatures around 1 K. The limit of zero temperature is also studied using the diffusion Monte Carlo method. Results for the energy, condensate fraction, and structure of the metastable liquid phase at T = 0 are reported and compared with the ones obtained for the stable solid phase.
ISSN:1098-0121
1550-235X
DOI:10.1103/PhysRevB.85.224513