Difference frequency generation by optical rectification of femtosecond laser pulse in GaAs crystal with a periodic domain structure

We study the influence of spatial boundedness of a femtosecond laser pulse (FLP) on the efficiency of generation of difference frequency radiation (DFR) in a GaAs crystal with a periodic domain structure. It is shown that at propagation of DFR a spectral-angular filtration occurs in the transverse distribution of the beam. An expression is obtained for the frequency-angular spectrum of DFR. For a pump pulse with the duration of 100 fs, the beam radius of 24μm, the energy of 30 nJ, and the wavelength of 1.98μm propagating in 1.716-mm long GaAs crystal with the domain structure period of 74.6μm the efficiency of generation of DFR at the wavelength of 14μm is calculated to be close to 2×10 −6 .