Nanosecond parametric Raman anti-Stokes SrWO 4 laser at 507 nm with collinear phase matching

Collinear phase matching of the Stokes ↔ anti-Stokes interaction for Raman-active crystals with different birefringence was studied theoretically as well as experimentally. It was shown that collinear phase matching of the Stokes ↔ anti-Stokes interaction in low-birefringent crystals can be insensitive to angular mismatch if a phase matching angle is higher than 60 ° . We have developed and experimentally realized an extracavity parametric Raman anti-Stokes laser based on a low-birefringent SrWO 4 . Cyan 507-nm anti-Stokes conversion from green (532 nm) pump radiation of a 5-ns, 1-mJ second harmonic Nd:YAG laser has been obtained. Laser setup with a single beam excitation made it possible to use an output face of the SrWO 4 crystal as an output coupler because of wide (6 ° ) angular tolerance of collinear phase matching that resulted in an increase of slope efficiency of anti-Stokes generation higher than 3% at the anti-Stokes energy output of a 10-µJ level.