Order and disorder in hard-sphere packings

We study the crystallisation of hard-sphere systems and compare the resulting packings with packings belonging to the stable branch of the phase diagram. This comparison is done by studying the distribution of a local bond order parameter which gives precise information on the structure and allows t...

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Veröffentlicht in:Europhysics letters 1999-11, Vol.48 (4), p.415-420
Hauptverfasser: Richard, P, Gervois, A, Oger, L, Troadec, J.-P
Format: Artikel
Sprache:eng
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Zusammenfassung:We study the crystallisation of hard-sphere systems and compare the resulting packings with packings belonging to the stable branch of the phase diagram. This comparison is done by studying the distribution of a local bond order parameter which gives precise information on the structure and allows to detect without ambiguity the presence of fcc or hcp crystallisation in the packing. We have found, as expected, that the fcc symmetry is more stable than the hcp symmetry in crystallised systems. Furthermore, the fraction of hcp clusters in the system decreases as the propensity to crystallise increases. The method developed here for hard-sphere systems can be applied to any kind of soft-sphere potential systems.
ISSN:0295-5075
1286-4854
DOI:10.1209/epl/i1999-00499-9