TiO 2 -SiO 2 supported MnWO x catalysts by liquid-phase deposition for low-temperature NH 3 -SCR
NH -SCR is an environmentally important reaction for the abatement of NO from different resources. MnO -based catalyst has attracted significant attention due to the excellent activity. In this paper, a series of MnWO /TiO -SiO catalysts were prepared by liquid-phase deposition method. The catalysts...
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creator | Lu, Weizhe Lu, Hanfeng Zhang, Zekai |
description | NH
-SCR is an environmentally important reaction for the abatement of NO
from different resources. MnO
-based catalyst has attracted significant attention due to the excellent activity. In this paper, a series of MnWO
/TiO
-SiO
catalysts were prepared by liquid-phase deposition method. The catalysts were characterized by N
adsorption/desorption, XRD, TEM, XPS, FT-IR, H
-TPR, TG and water adsorption capacity. The existence of SiO
improved the SO
and H
O resistance of the MnWO
/TiO
-SiO
catalyst without decreasing the NH
-SCR activity. Under the reaction conditions of 260°C and 60 000 ml g
h
gas hourly space velocity (GHSV), the NO conversion was kept stable at about 95% for 140 min on stream. The excellent performance of MnWO
/TiO
-SiO
catalyst is considered to be originated from the texture properties and active species dispersion improvement by SiO
in the support and low-temperature preparation. |
doi_str_mv | 10.1098/rsos.180669 |
format | Article |
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-SCR is an environmentally important reaction for the abatement of NO
from different resources. MnO
-based catalyst has attracted significant attention due to the excellent activity. In this paper, a series of MnWO
/TiO
-SiO
catalysts were prepared by liquid-phase deposition method. The catalysts were characterized by N
adsorption/desorption, XRD, TEM, XPS, FT-IR, H
-TPR, TG and water adsorption capacity. The existence of SiO
improved the SO
and H
O resistance of the MnWO
/TiO
-SiO
catalyst without decreasing the NH
-SCR activity. Under the reaction conditions of 260°C and 60 000 ml g
h
gas hourly space velocity (GHSV), the NO conversion was kept stable at about 95% for 140 min on stream. The excellent performance of MnWO
/TiO
-SiO
catalyst is considered to be originated from the texture properties and active species dispersion improvement by SiO
in the support and low-temperature preparation.</description><identifier>ISSN: 2054-5703</identifier><identifier>EISSN: 2054-5703</identifier><identifier>DOI: 10.1098/rsos.180669</identifier><identifier>PMID: 30800339</identifier><language>eng</language><publisher>England</publisher><ispartof>Royal Society open science, 2019-01, Vol.6 (1), p.180669</ispartof><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c1389-e66ff48cb6d98cf78d573fc5105029e9b534aefbbb593d1ea35dc61dcc7e6a163</citedby><cites>FETCH-LOGICAL-c1389-e66ff48cb6d98cf78d573fc5105029e9b534aefbbb593d1ea35dc61dcc7e6a163</cites><orcidid>0000-0002-4136-5263</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>315,782,786,866,3326,27933,27934</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/30800339$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Lu, Weizhe</creatorcontrib><creatorcontrib>Lu, Hanfeng</creatorcontrib><creatorcontrib>Zhang, Zekai</creatorcontrib><title>TiO 2 -SiO 2 supported MnWO x catalysts by liquid-phase deposition for low-temperature NH 3 -SCR</title><title>Royal Society open science</title><addtitle>R Soc Open Sci</addtitle><description>NH
-SCR is an environmentally important reaction for the abatement of NO
from different resources. MnO
-based catalyst has attracted significant attention due to the excellent activity. In this paper, a series of MnWO
/TiO
-SiO
catalysts were prepared by liquid-phase deposition method. The catalysts were characterized by N
adsorption/desorption, XRD, TEM, XPS, FT-IR, H
-TPR, TG and water adsorption capacity. The existence of SiO
improved the SO
and H
O resistance of the MnWO
/TiO
-SiO
catalyst without decreasing the NH
-SCR activity. Under the reaction conditions of 260°C and 60 000 ml g
h
gas hourly space velocity (GHSV), the NO conversion was kept stable at about 95% for 140 min on stream. The excellent performance of MnWO
/TiO
-SiO
catalyst is considered to be originated from the texture properties and active species dispersion improvement by SiO
in the support and low-temperature preparation.</description><issn>2054-5703</issn><issn>2054-5703</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2019</creationdate><recordtype>article</recordtype><recordid>eNpNkEtPAjEYRRujEYKs3JvuTfErpZ12aYiKCUqiGJdjn3HMwNR2Jsq_F0SNq3sXJ2dxEDqlMKKg5EXKTR5RCUKoA9QfA58QXgA7_Pd7aJjzGwBQDqwQxTHqMZAAjKk-ellWCzzG5PF7chdjk1rv8N36eYE_sdWtrje5zdhscF29d5Uj8VVnj52PTa7aqlnj0CRcNx-k9avok2675PH9DLOtdfpwgo6CrrMf_uwAPV1fLaczMl_c3E4v58RSJhXxQoQwkdYIp6QNhXS8YMFyChzGyivD2UT7YIzhijnqNePOCuqsLbzQVLABOt97bWpyTj6UMVUrnTYlhXKXqtylKveptvTZno6dWXn3x_6GYV-peGQC</recordid><startdate>201901</startdate><enddate>201901</enddate><creator>Lu, Weizhe</creator><creator>Lu, Hanfeng</creator><creator>Zhang, Zekai</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-4136-5263</orcidid></search><sort><creationdate>201901</creationdate><title>TiO 2 -SiO 2 supported MnWO x catalysts by liquid-phase deposition for low-temperature NH 3 -SCR</title><author>Lu, Weizhe ; Lu, Hanfeng ; Zhang, Zekai</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c1389-e66ff48cb6d98cf78d573fc5105029e9b534aefbbb593d1ea35dc61dcc7e6a163</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2019</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Lu, Weizhe</creatorcontrib><creatorcontrib>Lu, Hanfeng</creatorcontrib><creatorcontrib>Zhang, Zekai</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><jtitle>Royal Society open science</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Lu, Weizhe</au><au>Lu, Hanfeng</au><au>Zhang, Zekai</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>TiO 2 -SiO 2 supported MnWO x catalysts by liquid-phase deposition for low-temperature NH 3 -SCR</atitle><jtitle>Royal Society open science</jtitle><addtitle>R Soc Open Sci</addtitle><date>2019-01</date><risdate>2019</risdate><volume>6</volume><issue>1</issue><spage>180669</spage><pages>180669-</pages><issn>2054-5703</issn><eissn>2054-5703</eissn><abstract>NH
-SCR is an environmentally important reaction for the abatement of NO
from different resources. MnO
-based catalyst has attracted significant attention due to the excellent activity. In this paper, a series of MnWO
/TiO
-SiO
catalysts were prepared by liquid-phase deposition method. The catalysts were characterized by N
adsorption/desorption, XRD, TEM, XPS, FT-IR, H
-TPR, TG and water adsorption capacity. The existence of SiO
improved the SO
and H
O resistance of the MnWO
/TiO
-SiO
catalyst without decreasing the NH
-SCR activity. Under the reaction conditions of 260°C and 60 000 ml g
h
gas hourly space velocity (GHSV), the NO conversion was kept stable at about 95% for 140 min on stream. The excellent performance of MnWO
/TiO
-SiO
catalyst is considered to be originated from the texture properties and active species dispersion improvement by SiO
in the support and low-temperature preparation.</abstract><cop>England</cop><pmid>30800339</pmid><doi>10.1098/rsos.180669</doi><orcidid>https://orcid.org/0000-0002-4136-5263</orcidid><oa>free_for_read</oa></addata></record> |
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source | DOAJ Directory of Open Access Journals; Royal Society Open Access Journals; PubMed Central Open Access; EZB-FREE-00999 freely available EZB journals; PubMed Central |
title | TiO 2 -SiO 2 supported MnWO x catalysts by liquid-phase deposition for low-temperature NH 3 -SCR |
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