Tagged-particle motion in quasi-confined colloidal hard-sphere liquids
We investigate the tagged-particle motion in a strongly interacting quasi-confined liquid using periodic boundary conditions along the confining direction. Within a mode-coupling theory of the glass transition we calculate the self-nonergodicity parameters and the self-intermediate scattering functi...
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Veröffentlicht in: | Journal of statistical mechanics 2021-04, Vol.2021 (4), p.43301 |
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Hauptverfasser: | , , , , |
Format: | Artikel |
Sprache: | eng |
Online-Zugang: | Volltext |
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Zusammenfassung: | We investigate the tagged-particle motion in a strongly interacting quasi-confined liquid using periodic boundary conditions along the confining direction. Within a mode-coupling theory of the glass transition we calculate the self-nonergodicity parameters and the self-intermediate scattering function and compare them with event-driven molecular dynamics simulations. We observe non-monotonic behavior for the in-plane mean-square displacement and further correlation functions which refer to higher mode indices encoding information about the perpendicular motion. The in-plane velocity-autocorrelation function reveals persistent anti-correlations with a negative algebraic power-law decay
t
−2
at all packing fractions. |
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ISSN: | 1742-5468 1742-5468 |
DOI: | 10.1088/1742-5468/abee23 |