Experimental evidence of the oscillation behavior of the interlayer DMI effect

Chiral spin interactions play an important role in magnetism. Recent reports have revealed a new type of antisymmetric and indirect spin interaction, namely, the interlayer Dzyaloshinskii–Moriya interaction (DMI), which is predicted to arise from the three-site spin–orbit scattering of delocalized electrons as an additional Ruderman–Kittel–Kasuya–Yosida (RKKY) effect. Here, we investigated the interlayer DMI and RKKY interaction in the similar Pt/Co/Pt/Ru/Pt/Co/Pt structures as a function of spacer thickness. Both interactions present a synchronous damping oscillation and support the predicted relevance between them. The coupling strength of the interlayer DMI was finely engineered by tunning thickness of the nonmagnetic spacer. This work can deepen the understanding of the interlayer DMI and guide the control and use of the interlayer DMI in the field-free spin–orbit torque switching or the design of three-dimensional chiral spin textures.