High-pressure chemistry of hydrocarbons relevant to planetary interiors and inertial confinement fusion

Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606–611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations o...

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Veröffentlicht in:Physics of plasmas 2018-05, Vol.25 (5)
Hauptverfasser: Kraus, D., Hartley, N. J., Frydrych, S., Schuster, A. K., Rohatsch, K., Rödel, M., Cowan, T. E., Brown, S., Cunningham, E., van Driel, T., Fletcher, L. B., Galtier, E., Gamboa, E. J., Laso Garcia, A., Gericke, D. O., Granados, E., Heimann, P. A., Lee, H. J., MacDonald, M. J., MacKinnon, A. J., McBride, E. E., Nam, I., Neumayer, P., Pak, A., Pelka, A., Prencipe, I., Ravasio, A., Redmer, R., Saunders, A. M., Schölmerich, M., Schörner, M., Sun, P., Turner, S. J., Zettl, A., Falcone, R. W., Glenzer, S. H., Döppner, T., Vorberger, J.
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Sprache:eng
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Zusammenfassung:Diamond formation in polystyrene (C8H8)n, which is laser-compressed and heated to conditions around 150 GPa and 5000 K, has recently been demonstrated in the laboratory [Kraus et al., Nat. Astron. 1, 606–611 (2017)]. Here, we show an extended analysis and comparison to first-principles simulations of the acquired data and their implications for planetary physics and inertial confinement fusion. Moreover, we discuss the advanced diagnostic capabilities of adding high-quality small angle X-ray scattering and spectrally resolved X-ray scattering to the platform, which shows great prospects of precisely studying the kinetics of chemical reactions in dense plasma environments at pressures exceeding 100 GPa.
ISSN:1070-664X
1089-7674
DOI:10.1063/1.5017908