Invariant surfaces and phase space flux in three-dimensional surface diffusion

Investigation of the classical three-dimensional motion of a helium atom on a (001) xenon surface uncovered new invariant manifolds that are in close accord with recent theoretical developments in nonlinear dynamics. The relationship between these manifolds, phase space flux, and recrossing in trans...

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Veröffentlicht in:	The Journal of chemical physics 1990-10, Vol.93 (7), p.5300-5314
1. Verfasser:	GILLILAN, R. E
Format:	Artikel
Sprache:	eng
Schlagworte:	Condensed matter: structure, mechanical and thermal properties Exact sciences and technology Physics Solid surfaces and solid-solid interfaces Surface structure and topography Surfaces and interfaces thin films and whiskers (structure and nonelectronic properties)
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Beschreibung
Zusammenfassung:	Investigation of the classical three-dimensional motion of a helium atom on a (001) xenon surface uncovered new invariant manifolds that are in close accord with recent theoretical developments in nonlinear dynamics. The relationship between these manifolds, phase space flux, and recrossing in transition-state theory is explored. General theory and computational methods are also discussed.
ISSN:	0021-9606 1089-7690
DOI:	10.1063/1.459649