Double-impurity doping-induced quantum critical behaviors in Sr1−xBaxTi1−yRuyO3

It has been reported both experimentally and theoretically that the Ba2+-doping at the A-site of quantum paraelectric SrTiO3 suppresses the quantum fluctuations by activating the ferroelectric mode, while the Ru4+-doping at the B-site plays the opposite role. For a double-impurity doped SrTiO3, i.e....

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Veröffentlicht in:Journal of applied physics 2010-04, Vol.107 (7)
Hauptverfasser: Guo, Y. J., Wei, T., Zhu, C., Wang, K. F., Gao, X. S., Guan, Y. Q., Liu, J.-M.
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Sprache:eng
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Zusammenfassung:It has been reported both experimentally and theoretically that the Ba2+-doping at the A-site of quantum paraelectric SrTiO3 suppresses the quantum fluctuations by activating the ferroelectric mode, while the Ru4+-doping at the B-site plays the opposite role. For a double-impurity doped SrTiO3, i.e., Sr1−xBaxTi1−yRuyO3, where the two types of opposite effects compete with each other, we propose an improved transverse-field Ising model in order to investigate the effect of the double-impurity doping on the quantum phase transitions and critical behaviors. The calculated quantum behavior is quite well consistent with experimental measurements. A linear relationship between the quantum critical doping concentrations for Ba2+ and Ru4+ is predicted, subsequently validated qualitatively by an anharmonic oscillator model.
ISSN:0021-8979
1089-7550
DOI:10.1063/1.3361080