Giant changes in atomic dynamics on microalloying metallic melt

We report unexpectedly strong variations in the relaxational dynamics in a glass-forming metallic melt while microalloying. Analysis of quasielastic neutron scattering data revealed that changes in the values of stretching of the self-correlation function and the temperature dependence of self-diffu...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Applied physics letters 2009-11, Vol.95 (19), p.191907-191907-3
Hauptverfasser: Chathoth, S. M., Damaschke, B., Embs, J. P., Samwer, K.
Format: Artikel
Sprache:eng
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:We report unexpectedly strong variations in the relaxational dynamics in a glass-forming metallic melt while microalloying. Analysis of quasielastic neutron scattering data revealed that changes in the values of stretching of the self-correlation function and the temperature dependence of self-diffusivity showed an Arrhenius to non-Arrhenius transition. The intermediate structure of the melts did not show any prepeak or indication of short range order. These observations are correlated with the enhanced glass-forming ability of metallic melts on microalloying.
ISSN:0003-6951
1077-3118
DOI:10.1063/1.3263950