Femtosecond dephasing in porous silicon

We determine dephasing times T2 in free standing porous silicon samples using nondegenerate four-wave mixing. Within the framework of an idealized inhomogeneously broadened two-level system, values of 20 fs for different porosities are obtained. Fast energy relaxation times are found in the range of...

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Veröffentlicht in:Applied physics letters 1996-06, Vol.68 (23), p.3296-3298
Hauptverfasser: Tomasiunas, R., Moniatte, J., Pelant, I., Gilliot, P., Hönerlage, B.
Format: Artikel
Sprache:eng
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Zusammenfassung:We determine dephasing times T2 in free standing porous silicon samples using nondegenerate four-wave mixing. Within the framework of an idealized inhomogeneously broadened two-level system, values of 20 fs for different porosities are obtained. Fast energy relaxation times are found in the range of 1.5–3.5 ps for 64%–73% porosities, respectively. They are attributed to carrier thermalization within the band tails, originating from porous silicon nanocrystallites and their surface states.
ISSN:0003-6951
1077-3118
DOI:10.1063/1.116579