Metal– and covalent organic frameworks for photocatalytic CO 2 reduction coupled with H 2 O oxidation
The overuse of fossil fuels has caused serious energy and environmental issues. To address this, the integration of photocatalytic CO 2 reduction with H 2 O oxidation is considered an effective approach towards achieving carbon neutrality and sustainable development. This article presents a comprehe...
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Veröffentlicht in: | Inorganic chemistry frontiers 2024-05, Vol.11 (10), p.2819-2840 |
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creator | Zhou, Xiao-Xiang Ye, Yongshi Lin, Qia-Chun Liao, Wei-Ming He, Jun |
description | The overuse of fossil fuels has caused serious energy and environmental issues. To address this, the integration of photocatalytic CO
2
reduction with H
2
O oxidation is considered an effective approach towards achieving carbon neutrality and sustainable development. This article presents a comprehensive overview of the recent advancements in utilizing metal– and covalent organic frameworks for photocatalytic CO
2
reduction coupled with H
2
O oxidation. It discusses the key factors influencing the overall reaction, delves into the catalytic mechanisms of CO
2
reduction and H
2
O oxidation half-reactions, and explores the intermediate species involved in the process. Additionally, it summarizes various strategies employed by researchers to enhance the performance and product selectivity for the overall reaction. This review concludes with an outlook on the prospects and challenges of this emerging research field. |
doi_str_mv | 10.1039/D4QI00304G |
format | Article |
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2
reduction with H
2
O oxidation is considered an effective approach towards achieving carbon neutrality and sustainable development. This article presents a comprehensive overview of the recent advancements in utilizing metal– and covalent organic frameworks for photocatalytic CO
2
reduction coupled with H
2
O oxidation. It discusses the key factors influencing the overall reaction, delves into the catalytic mechanisms of CO
2
reduction and H
2
O oxidation half-reactions, and explores the intermediate species involved in the process. Additionally, it summarizes various strategies employed by researchers to enhance the performance and product selectivity for the overall reaction. This review concludes with an outlook on the prospects and challenges of this emerging research field.</description><identifier>ISSN: 2052-1553</identifier><identifier>EISSN: 2052-1553</identifier><identifier>DOI: 10.1039/D4QI00304G</identifier><language>eng</language><ispartof>Inorganic chemistry frontiers, 2024-05, Vol.11 (10), p.2819-2840</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-crossref_primary_10_1039_D4QI00304G3</cites><orcidid>0000-0001-7062-4001 ; 0000-0001-7799-0995</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids></links><search><creatorcontrib>Zhou, Xiao-Xiang</creatorcontrib><creatorcontrib>Ye, Yongshi</creatorcontrib><creatorcontrib>Lin, Qia-Chun</creatorcontrib><creatorcontrib>Liao, Wei-Ming</creatorcontrib><creatorcontrib>He, Jun</creatorcontrib><title>Metal– and covalent organic frameworks for photocatalytic CO 2 reduction coupled with H 2 O oxidation</title><title>Inorganic chemistry frontiers</title><description>The overuse of fossil fuels has caused serious energy and environmental issues. To address this, the integration of photocatalytic CO
2
reduction with H
2
O oxidation is considered an effective approach towards achieving carbon neutrality and sustainable development. This article presents a comprehensive overview of the recent advancements in utilizing metal– and covalent organic frameworks for photocatalytic CO
2
reduction coupled with H
2
O oxidation. It discusses the key factors influencing the overall reaction, delves into the catalytic mechanisms of CO
2
reduction and H
2
O oxidation half-reactions, and explores the intermediate species involved in the process. Additionally, it summarizes various strategies employed by researchers to enhance the performance and product selectivity for the overall reaction. This review concludes with an outlook on the prospects and challenges of this emerging research field.</description><issn>2052-1553</issn><issn>2052-1553</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNqVj01qAkEQhZugEFE3nqDWAZPq-QlkbaJmESTgfih6erR1nBqq24zuvENumJM4gqDbrN6D732Lp9RI47PG-O3lPfn-RIwxmT2oXoRpNNZpGnfu-qMaer9BRK0T1K_YU6svG6j8O_0CVTkY_qHSVgFYVlQ5A4XQzjYsWw8FC9RrDmyoNY6hpZMFRCA235vguGrtfV3aHBoX1jBv0QL44HK6wIHqFlR6O7xmXz1NP5aT-dgIey-2yGpxO5JjpjG7vMlub-J_jc8T9lDM</recordid><startdate>20240514</startdate><enddate>20240514</enddate><creator>Zhou, Xiao-Xiang</creator><creator>Ye, Yongshi</creator><creator>Lin, Qia-Chun</creator><creator>Liao, Wei-Ming</creator><creator>He, Jun</creator><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-7062-4001</orcidid><orcidid>https://orcid.org/0000-0001-7799-0995</orcidid></search><sort><creationdate>20240514</creationdate><title>Metal– and covalent organic frameworks for photocatalytic CO 2 reduction coupled with H 2 O oxidation</title><author>Zhou, Xiao-Xiang ; Ye, Yongshi ; Lin, Qia-Chun ; Liao, Wei-Ming ; He, Jun</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-crossref_primary_10_1039_D4QI00304G3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhou, Xiao-Xiang</creatorcontrib><creatorcontrib>Ye, Yongshi</creatorcontrib><creatorcontrib>Lin, Qia-Chun</creatorcontrib><creatorcontrib>Liao, Wei-Ming</creatorcontrib><creatorcontrib>He, Jun</creatorcontrib><collection>CrossRef</collection><jtitle>Inorganic chemistry frontiers</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhou, Xiao-Xiang</au><au>Ye, Yongshi</au><au>Lin, Qia-Chun</au><au>Liao, Wei-Ming</au><au>He, Jun</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Metal– and covalent organic frameworks for photocatalytic CO 2 reduction coupled with H 2 O oxidation</atitle><jtitle>Inorganic chemistry frontiers</jtitle><date>2024-05-14</date><risdate>2024</risdate><volume>11</volume><issue>10</issue><spage>2819</spage><epage>2840</epage><pages>2819-2840</pages><issn>2052-1553</issn><eissn>2052-1553</eissn><abstract>The overuse of fossil fuels has caused serious energy and environmental issues. To address this, the integration of photocatalytic CO
2
reduction with H
2
O oxidation is considered an effective approach towards achieving carbon neutrality and sustainable development. This article presents a comprehensive overview of the recent advancements in utilizing metal– and covalent organic frameworks for photocatalytic CO
2
reduction coupled with H
2
O oxidation. It discusses the key factors influencing the overall reaction, delves into the catalytic mechanisms of CO
2
reduction and H
2
O oxidation half-reactions, and explores the intermediate species involved in the process. Additionally, it summarizes various strategies employed by researchers to enhance the performance and product selectivity for the overall reaction. This review concludes with an outlook on the prospects and challenges of this emerging research field.</abstract><doi>10.1039/D4QI00304G</doi><orcidid>https://orcid.org/0000-0001-7062-4001</orcidid><orcidid>https://orcid.org/0000-0001-7799-0995</orcidid></addata></record> |
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source | Royal Society Of Chemistry Journals 2008- |
title | Metal– and covalent organic frameworks for photocatalytic CO 2 reduction coupled with H 2 O oxidation |
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