Magnetocaloric effect and critical behavior of the La 0.75 Ca 0.1 Na 0.15 MnO 3 compound

In this paper, we have studied the critical behavior and the magnetocaloric effect (MCE) simulation for the La Ca Na MnO (LCNMO) compound at the second order ferromagnetic-paramagnetic phase transition. The optimized critical exponents, based on the Kouvel-Fisher method, were found to be: = 0.48 and...

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Veröffentlicht in:RSC advances 2023-05, Vol.13 (24), p.16529-16535
Hauptverfasser: Bouzidi, Souhir, Hsini, Mohamed, Soltani, Sonia, Essid, Manel, Albedah, M A, Belmabrouk, Hafedh, Dhahri, J
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Sprache:eng
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Zusammenfassung:In this paper, we have studied the critical behavior and the magnetocaloric effect (MCE) simulation for the La Ca Na MnO (LCNMO) compound at the second order ferromagnetic-paramagnetic phase transition. The optimized critical exponents, based on the Kouvel-Fisher method, were found to be: = 0.48 and = 1. These obtained values supposed that the Mean Field Model (MFM) is the proper model to analyze adequately the MCE in the LCNMO sample. The isothermal magnetization ( , ) and the magnetic entropy change -Δ ( , ) curves were successfully simulated using three models, namely the Arrott-Noakes equation (ANE) of state, Landau theory, and MFM. The framework of the MFM allows us to estimate magnetic entropy variation in a wide temperature range within the thermodynamics of the model and without using the usual numerical integration of Maxwell relation.
ISSN:2046-2069
2046-2069
DOI:10.1039/D3RA02443A