Self-regulating electrical rhythms with liquid crystal oligomer networks in hybrid circuitry

Self-regulation is an essential aspect in the practicality of electronic systems, ranging from household heaters to robots for industrial manufacturing. In such devices, self-regulation is conventionally achieved through separate sensors working in tandem with control modules. In this paper, we harness the reversible actuating properties of liquid crystal oligomer network (LCON) polymers to design a self-regulated oscillator. A dynamic equilibrium is achieved by applying a thermally-responsive and electrically-functionalized LCON film as a dual-action component, namely as a combined electrical switch and composite actuating sensor, within a circuit. This hybrid circuit configuration, consisting of both inorganic and organic material, generates a self-regulated feedback loop which cycles regularly and indefinitely. The feedback loop cycle frequency is tunable between approximately 0.08 and 0.87 Hz by altering multiple factors, such as supplied power or LCON chemistry. Our research aims to drive the material-to-device transition of stimuli-responsive LCONs, striving towards applications in electronic soft robotics. Self-regulation in liquid crystal systems marks an important step towards harnessing its advanced soft robotic functions.