Photocapacitor integrating voltage-adjustable hybrid supercapacitor and silicon solar cell generating a Joule efficiency of 86

Photocapacitor integrating both energy harvest and storage functions into a single device is a frontier research orientation, which facilitates the efficient and sustainable utilization of green energy. However, the multi-functions in one device and structural complexity of the integrated device, pa...

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Veröffentlicht in:Energy & environmental science 2022-10, Vol.15 (1), p.4247-4258
Hauptverfasser: Song, Zeyu, Wu, Jihuai, Tu, Yongguang, Sun, Liuxue, Zhu, Tingting, Li, Guodong, Wang, Xiaobing, Du, Yitian, Deng, Chunyan, Chen, Qi, Sun, Weihai, Huang, Miaoliang, Fan, Leqing, Huang, Yunfang, Wei, Yuelin, Xie, Yiming, Lin, Yu, Chen, Hongwei, Lin, Jianming, Zhan, Lan, Gao, Peng, Nazeeruddin, Mohammad Khaja, Huang, Wei
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container_issue 1
container_start_page 4247
container_title Energy & environmental science
container_volume 15
creator Song, Zeyu
Wu, Jihuai
Tu, Yongguang
Sun, Liuxue
Zhu, Tingting
Li, Guodong
Wang, Xiaobing
Du, Yitian
Deng, Chunyan
Chen, Qi
Sun, Weihai
Huang, Miaoliang
Fan, Leqing
Huang, Yunfang
Wei, Yuelin
Xie, Yiming
Lin, Yu
Chen, Hongwei
Lin, Jianming
Zhan, Lan
Gao, Peng
Nazeeruddin, Mohammad Khaja
Huang, Wei
description Photocapacitor integrating both energy harvest and storage functions into a single device is a frontier research orientation, which facilitates the efficient and sustainable utilization of green energy. However, the multi-functions in one device and structural complexity of the integrated device, particularly the mismatch between energy harvest and storage units, lead to a relatively large energy loss in the energy storage and output processes. Here, we design a voltage adjustable hybrid supercapacitor (VAHSC) as an energy storage unit of a three-terminal photocapacitor. The VAHSC effectively harmonizes the energy harvest and storage units, resulting in the current, voltage, power, and energy match between both units. The optimal photocapacitor achieves a storage efficiency as high as 98.28% and Joule efficiency of 86.01%, along with excellent charge/discharge cycle stability. The great leap in this efficiency marks a substantial step towards the practical application of solar-charging energy storage integrated devices. Photocapacitor integrating both energy harvest and storage functions into a single device is a frontier research orientation, which facilitates the efficient and sustainable utilization of green energy.
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source Royal Society Of Chemistry Journals 2008-
subjects Clean energy
Electric potential
Energy harvesting
Energy loss
Energy storage
Photocapacitors
Photovoltaic cells
Renewable energy
Solar cells
Solar energy
Storage units
Supercapacitors
Voltage
title Photocapacitor integrating voltage-adjustable hybrid supercapacitor and silicon solar cell generating a Joule efficiency of 86
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