Sequential energy transfer followed by electron transfer in a BODIPY-bisstyrylBODIPY bound to C 60 triad via a 'two-point' binding strategy

Sequential energy transfer followed by electron transfer in a BODIPY-bisstyrylBODIPY bound to C 60 triad via a 'two-point' binding strategy

Excitation transfer from BODIPY* to bisstyrylBODIPY followed by electron transfer to C leading to a charge separated state of appreciable lifetime in a supramolecularly assembled triad is demonstrated, as a mimic of the photosynthetic 'antenna-reaction centre'.

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Veröffentlicht in:Chemical communications (Cambridge, England) England), 2018-01, Vol.54 (1), p.54-57
Hauptverfasser: Shao, Shuai, Thomas, Michael B, Park, Kyu Hyung, Mahaffey, Zoe, Kim, Dongho, D'Souza, Francis
Format: Artikel
Sprache:eng
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Zusammenfassung:Excitation transfer from BODIPY* to bisstyrylBODIPY followed by electron transfer to C leading to a charge separated state of appreciable lifetime in a supramolecularly assembled triad is demonstrated, as a mimic of the photosynthetic 'antenna-reaction centre'.
ISSN:1359-7345
1364-548X
DOI:10.1039/c7cc08063h