A highly photoactive, visible-light-driven graphene/2D mesoporous TiO 2 photocatalyst

In this paper, we have reported a new, visible-light-driven photocatalyst composed of 2D mesoporous TiO 2 on reduced graphene oxide, which enables enhanced absorption of visible light, showing outstanding charge separation ability and a large surface area. Graphene–2D mesoporous TiO 2 (GOMTi) was pr...

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Veröffentlicht in:Green chemistry : an international journal and green chemistry resource : GC 2015, Vol.17 (7), p.3972-3978
Hauptverfasser: Cho, Kyeong Min, Kim, Kyoung Hwan, Choi, Hyung Ouk, Jung, Hee-Tae
Format: Artikel
Sprache:eng
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Zusammenfassung:In this paper, we have reported a new, visible-light-driven photocatalyst composed of 2D mesoporous TiO 2 on reduced graphene oxide, which enables enhanced absorption of visible light, showing outstanding charge separation ability and a large surface area. Graphene–2D mesoporous TiO 2 (GOMTi) was prepared via a simple hydrothermal process by ternary self-assembly of metal oxide precursors, graphene oxide, and a surfactant. The structural strength and large interfacial contact between the graphene and two dimensional TiO 2 sheet lead to a high performance photocatalyst, as compared to a conventional graphene–TiO 2 nanostructure composite. In the test for degradation of methylene blue, the photodegradation rate of GOMTi was ∼9 times higher than the rate of common TiO 2 nanoparticles (p25), due to the enhanced synergetic effects of graphene and TiO 2 .
ISSN:1463-9262
1463-9270
DOI:10.1039/C5GC00641D