Sensitivity of NO x over the Indian Ocean to emissions from the surrounding continents and nonlinearities in atmospheric chemistry responses
The sensitivity of the Indian Ocean atmospheric chemistry to continental NO x emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO x responds nonlinearly to changes in emissions, since O 3 and OH, which depend on NO x , influence its lifetime. Due to this feedback and the...
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Veröffentlicht in: | Geophysical research letters 2004-08, Vol.31 (15) |
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creator | Kunhikrishnan, T. Lawrence, M. G. |
description | The sensitivity of the Indian Ocean atmospheric chemistry to continental NO
x
emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO
x
responds nonlinearly to changes in emissions, since O
3
and OH, which depend on NO
x
, influence its lifetime. Due to this feedback and the contribution from other NO
x
sources (e.g., lightning), much of the Indian Ocean lower troposphere (LT) is only weakly sensitive to continental NO
x
emissions. In contrast to INDOEX (Indian Ocean Experiment) results for aerosols, CO, etc., during the winter monsoon the central Indian Ocean (CIO) is weakly sensitivity to Indian NO
x
emissions. However, the Bay of Bengal LT is very sensitive to NO
x
emissions from India (summer) and SE Asia and China (winter). Higher up, NO
x
over the CIO is most sensitive to African and SE Asian emissions, while the northern regions are influenced by the summer monsoon plume from India, SE Asia and China. |
doi_str_mv | 10.1029/2004GL020210 |
format | Article |
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x
emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO
x
responds nonlinearly to changes in emissions, since O
3
and OH, which depend on NO
x
, influence its lifetime. Due to this feedback and the contribution from other NO
x
sources (e.g., lightning), much of the Indian Ocean lower troposphere (LT) is only weakly sensitive to continental NO
x
emissions. In contrast to INDOEX (Indian Ocean Experiment) results for aerosols, CO, etc., during the winter monsoon the central Indian Ocean (CIO) is weakly sensitivity to Indian NO
x
emissions. However, the Bay of Bengal LT is very sensitive to NO
x
emissions from India (summer) and SE Asia and China (winter). Higher up, NO
x
over the CIO is most sensitive to African and SE Asian emissions, while the northern regions are influenced by the summer monsoon plume from India, SE Asia and China.</description><identifier>ISSN: 0094-8276</identifier><identifier>EISSN: 1944-8007</identifier><identifier>DOI: 10.1029/2004GL020210</identifier><language>eng</language><ispartof>Geophysical research letters, 2004-08, Vol.31 (15)</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c800-40a5b2608c23f1c1a5d6e3001d0f6242ec327998fcc65185ed75c8bade3821213</citedby><cites>FETCH-LOGICAL-c800-40a5b2608c23f1c1a5d6e3001d0f6242ec327998fcc65185ed75c8bade3821213</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27923,27924</link.rule.ids></links><search><creatorcontrib>Kunhikrishnan, T.</creatorcontrib><creatorcontrib>Lawrence, M. G.</creatorcontrib><title>Sensitivity of NO x over the Indian Ocean to emissions from the surrounding continents and nonlinearities in atmospheric chemistry responses</title><title>Geophysical research letters</title><description>The sensitivity of the Indian Ocean atmospheric chemistry to continental NO
x
emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO
x
responds nonlinearly to changes in emissions, since O
3
and OH, which depend on NO
x
, influence its lifetime. Due to this feedback and the contribution from other NO
x
sources (e.g., lightning), much of the Indian Ocean lower troposphere (LT) is only weakly sensitive to continental NO
x
emissions. In contrast to INDOEX (Indian Ocean Experiment) results for aerosols, CO, etc., during the winter monsoon the central Indian Ocean (CIO) is weakly sensitivity to Indian NO
x
emissions. However, the Bay of Bengal LT is very sensitive to NO
x
emissions from India (summer) and SE Asia and China (winter). Higher up, NO
x
over the CIO is most sensitive to African and SE Asian emissions, while the northern regions are influenced by the summer monsoon plume from India, SE Asia and China.</description><issn>0094-8276</issn><issn>1944-8007</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2004</creationdate><recordtype>article</recordtype><recordid>eNpNkM1KA0EQhAdRMEZvPkA_gKs9M_t7lKAxEMzB3JfJbK8ZSWbC9CSYd_Ch3agHL9VVUHzQJcStxHuJqnlQiPl0jgqVxDMxkk2eZzVidS5GiM3gVVVeiivmD0TUqOVIfL2RZ5fcwaUjhB5eF_AJ4UAR0ppg5jtnPCwsDZoC0NYxu-AZ-hi2PxXexxj2Q8-_gw0-OU8-MRjfgQ9-M0QTBz4xOA8mbQPv1hSdBbs-0VI8QiTeDUzia3HRmw3Tzd8di-Xz03Lyks0X09nkcZ7Z4ZssR1OsVIm1VbqXVpqiK0kjyg77UuWKrFZV09S9tWUh64K6qrD1ynSkayWV1GNx94u1MTBH6ttddFsTj63E9jRk-39I_Q37Z2ig</recordid><startdate>200408</startdate><enddate>200408</enddate><creator>Kunhikrishnan, T.</creator><creator>Lawrence, M. G.</creator><scope>AAYXX</scope><scope>CITATION</scope></search><sort><creationdate>200408</creationdate><title>Sensitivity of NO x over the Indian Ocean to emissions from the surrounding continents and nonlinearities in atmospheric chemistry responses</title><author>Kunhikrishnan, T. ; Lawrence, M. G.</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c800-40a5b2608c23f1c1a5d6e3001d0f6242ec327998fcc65185ed75c8bade3821213</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2004</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Kunhikrishnan, T.</creatorcontrib><creatorcontrib>Lawrence, M. G.</creatorcontrib><collection>CrossRef</collection><jtitle>Geophysical research letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Kunhikrishnan, T.</au><au>Lawrence, M. G.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Sensitivity of NO x over the Indian Ocean to emissions from the surrounding continents and nonlinearities in atmospheric chemistry responses</atitle><jtitle>Geophysical research letters</jtitle><date>2004-08</date><risdate>2004</risdate><volume>31</volume><issue>15</issue><issn>0094-8276</issn><eissn>1944-8007</eissn><abstract>The sensitivity of the Indian Ocean atmospheric chemistry to continental NO
x
emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO
x
responds nonlinearly to changes in emissions, since O
3
and OH, which depend on NO
x
, influence its lifetime. Due to this feedback and the contribution from other NO
x
sources (e.g., lightning), much of the Indian Ocean lower troposphere (LT) is only weakly sensitive to continental NO
x
emissions. In contrast to INDOEX (Indian Ocean Experiment) results for aerosols, CO, etc., during the winter monsoon the central Indian Ocean (CIO) is weakly sensitivity to Indian NO
x
emissions. However, the Bay of Bengal LT is very sensitive to NO
x
emissions from India (summer) and SE Asia and China (winter). Higher up, NO
x
over the CIO is most sensitive to African and SE Asian emissions, while the northern regions are influenced by the summer monsoon plume from India, SE Asia and China.</abstract><doi>10.1029/2004GL020210</doi></addata></record> |
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title | Sensitivity of NO x over the Indian Ocean to emissions from the surrounding continents and nonlinearities in atmospheric chemistry responses |
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