Sensitivity of NO x over the Indian Ocean to emissions from the surrounding continents and nonlinearities in atmospheric chemistry responses
The sensitivity of the Indian Ocean atmospheric chemistry to continental NO x emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO x responds nonlinearly to changes in emissions, since O 3 and OH, which depend on NO x , influence its lifetime. Due to this feedback and the...
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Veröffentlicht in: | Geophysical research letters 2004-08, Vol.31 (15) |
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Hauptverfasser: | , |
Format: | Artikel |
Sprache: | eng |
Online-Zugang: | Volltext |
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Zusammenfassung: | The sensitivity of the Indian Ocean atmospheric chemistry to continental NO
x
emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO
x
responds nonlinearly to changes in emissions, since O
3
and OH, which depend on NO
x
, influence its lifetime. Due to this feedback and the contribution from other NO
x
sources (e.g., lightning), much of the Indian Ocean lower troposphere (LT) is only weakly sensitive to continental NO
x
emissions. In contrast to INDOEX (Indian Ocean Experiment) results for aerosols, CO, etc., during the winter monsoon the central Indian Ocean (CIO) is weakly sensitivity to Indian NO
x
emissions. However, the Bay of Bengal LT is very sensitive to NO
x
emissions from India (summer) and SE Asia and China (winter). Higher up, NO
x
over the CIO is most sensitive to African and SE Asian emissions, while the northern regions are influenced by the summer monsoon plume from India, SE Asia and China. |
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ISSN: | 0094-8276 1944-8007 |
DOI: | 10.1029/2004GL020210 |