Sensitivity of NO x over the Indian Ocean to emissions from the surrounding continents and nonlinearities in atmospheric chemistry responses

The sensitivity of the Indian Ocean atmospheric chemistry to continental NO x emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO x responds nonlinearly to changes in emissions, since O 3 and OH, which depend on NO x , influence its lifetime. Due to this feedback and the...

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Veröffentlicht in:Geophysical research letters 2004-08, Vol.31 (15)
Hauptverfasser: Kunhikrishnan, T., Lawrence, M. G.
Format: Artikel
Sprache:eng
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Zusammenfassung:The sensitivity of the Indian Ocean atmospheric chemistry to continental NO x emissions is examined using a global chemistry‐transport model (MATCH‐MPIC). NO x responds nonlinearly to changes in emissions, since O 3 and OH, which depend on NO x , influence its lifetime. Due to this feedback and the contribution from other NO x sources (e.g., lightning), much of the Indian Ocean lower troposphere (LT) is only weakly sensitive to continental NO x emissions. In contrast to INDOEX (Indian Ocean Experiment) results for aerosols, CO, etc., during the winter monsoon the central Indian Ocean (CIO) is weakly sensitivity to Indian NO x emissions. However, the Bay of Bengal LT is very sensitive to NO x emissions from India (summer) and SE Asia and China (winter). Higher up, NO x over the CIO is most sensitive to African and SE Asian emissions, while the northern regions are influenced by the summer monsoon plume from India, SE Asia and China.
ISSN:0094-8276
1944-8007
DOI:10.1029/2004GL020210