Enhanced Thermal Sensitivity of Silicon Nanoparticles Embedded in (Nano-Ag/)SiN x for Luminescent Thermometry

Steady-state photoluminescence of silicon nanoparticles embedded in solid-state (nano-Ag/)SiN x thin films at above room temperature is studied and compared to silicon nanoparticles dispersed in low-polar liquids. Roles of local surface plasmons as well as general mechanisms responsible for the temp...

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Veröffentlicht in:Journal of physical chemistry. C 2014-06, Vol.118 (23), p.12515-12519
Hauptverfasser: Ryabchikov, Yury V, Lysenko, Vladimir, Nychyporuk, Tetyana
Format: Artikel
Sprache:eng
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Zusammenfassung:Steady-state photoluminescence of silicon nanoparticles embedded in solid-state (nano-Ag/)SiN x thin films at above room temperature is studied and compared to silicon nanoparticles dispersed in low-polar liquids. Roles of local surface plasmons as well as general mechanisms responsible for the temperature-dependent photoluminescence are pointed out. Thermal sensitivities of photoluminescence spectral shape, maximum position, and full width at half-maximum are estimated and application of the (nano-Ag/)SiN x layers as photoluminescent thermal screens is proposed.
ISSN:1932-7447
1932-7455
DOI:10.1021/jp411887s