Hybrid Standing Wave and Whispering Gallery Modes in Needle-Shaped ZnO Rods: Simulation of Emission Microscopy Images Using Finite Difference Frequency Domain Methods with a Focused Gaussian Source

Two-photon emission microscopy is used to investigate the photoluminescence properties of individual ZnO rods. The rods are 10–20 μm in length with a tapered cross section that varies from 1 to 2 μm at the midpoint to several hundred nanometers at the ends. The tapered shape and hexagonal cross sect...

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Veröffentlicht in:Journal of physical chemistry. C 2013-05, Vol.117 (20), p.10653-10660
Hauptverfasser: Kirschbrown, Justin R, House, Ralph L, Mehl, Brian P, Parker, James K, Papanikolas, John M
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Sprache:eng
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Zusammenfassung:Two-photon emission microscopy is used to investigate the photoluminescence properties of individual ZnO rods. The rods are 10–20 μm in length with a tapered cross section that varies from 1 to 2 μm at the midpoint to several hundred nanometers at the ends. The tapered shape and hexagonal cross section result in complex optical resonator modes that lead to periodic patterns in the two-photon emission image. Finite-difference frequency domain methods using a series of excitation sources, including focused Gaussian, point dipole, and plane wave, suggest that resonator modes have both standing wave (Fabry-Pérot) and whispering gallery mode character, whose relative contributions vary along the rod axis.
ISSN:1932-7447
1932-7455
DOI:10.1021/jp4011907