Rationalizing an Unexpected Structure Sensitivity in Heterogeneous CatalysisCO Hydrogenation over Rh as a Case Study

A common expectation in heterogeneous catalysis is that the optimal activity will occur for the particle size with the highest concentration of undercoordinated step, edge, or corner sites, expectedly in the

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Veröffentlicht in:ACS catalysis 2021-05, Vol.11 (9), p.5189-5201
Hauptverfasser: Schumann, Max, Nielsen, Monia R, Smitshuysen, Thomas E. L, Hansen, Thomas W, Damsgaard, Christian D, Yang, An-Chih A, Cargnello, Matteo, Grunwaldt, Jan-Dierk, Jensen, Anker D, Christensen, Jakob M
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Sprache:eng
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Zusammenfassung:A common expectation in heterogeneous catalysis is that the optimal activity will occur for the particle size with the highest concentration of undercoordinated step, edge, or corner sites, expectedly in the
ISSN:2155-5435
2155-5435
DOI:10.1021/acscatal.0c05002