Self-Oriented Functionalized MXene with Excellent Antioxidant Properties for Enhancing Anticorrosion Properties of Waterborne Epoxy Resin
A MXene/poly(dimethyl diallyl ammonium chloride) (PDDA)/Fe3O4 (MPF) hybrid with exceptional oxidation resistance was synthesized via electrostatic self-assembly. Subsequently, a magnetic field was utilized to construct the parallel-aligned MPF within the waterborne epoxy coating (WEC). This paralle...
Gespeichert in:
| Veröffentlicht in: | Industrial & engineering chemistry research 2024-06, Vol.63 (24), p.10637-10650 |
|---|---|
| Hauptverfasser: | , , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 10650 |
|---|---|
| container_issue | 24 |
| container_start_page | 10637 |
| container_title | Industrial & engineering chemistry research |
| container_volume | 63 |
| creator | Fan, Yawen Wu, Jiongxin Zhang, Li Sheng, Xinxin |
| description | A MXene/poly(dimethyl diallyl ammonium chloride) (PDDA)/Fe3O4 (MPF) hybrid with exceptional oxidation resistance was synthesized via electrostatic self-assembly. Subsequently, a magnetic field was utilized to construct the parallel-aligned MPF within the waterborne epoxy coating (WEC). This parallel-aligned hybrid could significantly hinder the penetration of the corrosive ions. The electrochemical impedance spectroscopy (EIS) results revealed that the WEC containing parallel-aligned MPF (VMPF/WEC) exhibited the highest low-frequency impedance modulus (|Z 0.01 Hz|) among all coatings, which was 3 orders of magnitude higher than that of WEC in the initial stage of corrosion. After 42 days of the corrosion, the |Z 0.01 Hz| of VMPF/WEC surpassed that of WEC by more than 2 orders of magnitude, thereby indicating the exceptional long-term corrosion resistance of VMPF/WEC. This work proposed novel ideas for constructing high-performance anticorrosion WECs. |
| doi_str_mv | 10.1021/acs.iecr.4c01100 |
| format | Article |
| fullrecord | <record><control><sourceid>acs_cross</sourceid><recordid>TN_cdi_crossref_primary_10_1021_acs_iecr_4c01100</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>c254464385</sourcerecordid><originalsourceid>FETCH-LOGICAL-a210t-e1e2a79fc157eec2a16694d2200d1f4463168b13465fe2f107b49c7553c0ebc3</originalsourceid><addsrcrecordid>eNp1kMFOAjEQhhujiYjePe4DuDjttrvLkRBQEwxGSfS26XanUrK2pF0i-Aa-tUU4ePE0M5lv_kw-Qq4pDCgweitVGBhUfsAVUApwQnpUMEgFcHFKelCWZSrKUpyTixBWACAE5z3y_YKtTufeoO2wSaYbqzrjrGzNVxwf39Bi8mm6ZTLZKmzbSCUjG4mtaWTsn7xbo-8MhkQ7n0zsUlpl7PsvpJz3LsS0v5jTyavs0NfOx-jJ2m13yTMGYy_JmZZtwKtj7ZPFdLIY36ez-d3DeDRLJaPQpUiRyWKoFRUFomKS5vmQN4wBNFRznmc0L2ua8VxoZJpCUfOhKoTIFGCtsj6BQ6yKvwWPulp78yH9rqJQ7U1W0WS1N1kdTcaTm8PJfrNyGx_1hP_xH9NietE</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Self-Oriented Functionalized MXene with Excellent Antioxidant Properties for Enhancing Anticorrosion Properties of Waterborne Epoxy Resin</title><source>American Chemical Society Journals</source><creator>Fan, Yawen ; Wu, Jiongxin ; Zhang, Li ; Sheng, Xinxin</creator><creatorcontrib>Fan, Yawen ; Wu, Jiongxin ; Zhang, Li ; Sheng, Xinxin</creatorcontrib><description>A MXene/poly(dimethyl diallyl ammonium chloride) (PDDA)/Fe3O4 (MPF) hybrid with exceptional oxidation resistance was synthesized via electrostatic self-assembly. Subsequently, a magnetic field was utilized to construct the parallel-aligned MPF within the waterborne epoxy coating (WEC). This parallel-aligned hybrid could significantly hinder the penetration of the corrosive ions. The electrochemical impedance spectroscopy (EIS) results revealed that the WEC containing parallel-aligned MPF (VMPF/WEC) exhibited the highest low-frequency impedance modulus (|Z 0.01 Hz|) among all coatings, which was 3 orders of magnitude higher than that of WEC in the initial stage of corrosion. After 42 days of the corrosion, the |Z 0.01 Hz| of VMPF/WEC surpassed that of WEC by more than 2 orders of magnitude, thereby indicating the exceptional long-term corrosion resistance of VMPF/WEC. This work proposed novel ideas for constructing high-performance anticorrosion WECs.</description><identifier>ISSN: 0888-5885</identifier><identifier>EISSN: 1520-5045</identifier><identifier>DOI: 10.1021/acs.iecr.4c01100</identifier><language>eng</language><publisher>American Chemical Society</publisher><subject>Materials and Interfaces</subject><ispartof>Industrial & engineering chemistry research, 2024-06, Vol.63 (24), p.10637-10650</ispartof><rights>2024 American Chemical Society</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-a210t-e1e2a79fc157eec2a16694d2200d1f4463168b13465fe2f107b49c7553c0ebc3</citedby><cites>FETCH-LOGICAL-a210t-e1e2a79fc157eec2a16694d2200d1f4463168b13465fe2f107b49c7553c0ebc3</cites><orcidid>0000-0001-7695-0430</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/acs.iecr.4c01100$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/acs.iecr.4c01100$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,2765,27076,27924,27925,56738,56788</link.rule.ids></links><search><creatorcontrib>Fan, Yawen</creatorcontrib><creatorcontrib>Wu, Jiongxin</creatorcontrib><creatorcontrib>Zhang, Li</creatorcontrib><creatorcontrib>Sheng, Xinxin</creatorcontrib><title>Self-Oriented Functionalized MXene with Excellent Antioxidant Properties for Enhancing Anticorrosion Properties of Waterborne Epoxy Resin</title><title>Industrial & engineering chemistry research</title><addtitle>Ind. Eng. Chem. Res</addtitle><description>A MXene/poly(dimethyl diallyl ammonium chloride) (PDDA)/Fe3O4 (MPF) hybrid with exceptional oxidation resistance was synthesized via electrostatic self-assembly. Subsequently, a magnetic field was utilized to construct the parallel-aligned MPF within the waterborne epoxy coating (WEC). This parallel-aligned hybrid could significantly hinder the penetration of the corrosive ions. The electrochemical impedance spectroscopy (EIS) results revealed that the WEC containing parallel-aligned MPF (VMPF/WEC) exhibited the highest low-frequency impedance modulus (|Z 0.01 Hz|) among all coatings, which was 3 orders of magnitude higher than that of WEC in the initial stage of corrosion. After 42 days of the corrosion, the |Z 0.01 Hz| of VMPF/WEC surpassed that of WEC by more than 2 orders of magnitude, thereby indicating the exceptional long-term corrosion resistance of VMPF/WEC. This work proposed novel ideas for constructing high-performance anticorrosion WECs.</description><subject>Materials and Interfaces</subject><issn>0888-5885</issn><issn>1520-5045</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp1kMFOAjEQhhujiYjePe4DuDjttrvLkRBQEwxGSfS26XanUrK2pF0i-Aa-tUU4ePE0M5lv_kw-Qq4pDCgweitVGBhUfsAVUApwQnpUMEgFcHFKelCWZSrKUpyTixBWACAE5z3y_YKtTufeoO2wSaYbqzrjrGzNVxwf39Bi8mm6ZTLZKmzbSCUjG4mtaWTsn7xbo-8MhkQ7n0zsUlpl7PsvpJz3LsS0v5jTyavs0NfOx-jJ2m13yTMGYy_JmZZtwKtj7ZPFdLIY36ez-d3DeDRLJaPQpUiRyWKoFRUFomKS5vmQN4wBNFRznmc0L2ua8VxoZJpCUfOhKoTIFGCtsj6BQ6yKvwWPulp78yH9rqJQ7U1W0WS1N1kdTcaTm8PJfrNyGx_1hP_xH9NietE</recordid><startdate>20240619</startdate><enddate>20240619</enddate><creator>Fan, Yawen</creator><creator>Wu, Jiongxin</creator><creator>Zhang, Li</creator><creator>Sheng, Xinxin</creator><general>American Chemical Society</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0001-7695-0430</orcidid></search><sort><creationdate>20240619</creationdate><title>Self-Oriented Functionalized MXene with Excellent Antioxidant Properties for Enhancing Anticorrosion Properties of Waterborne Epoxy Resin</title><author>Fan, Yawen ; Wu, Jiongxin ; Zhang, Li ; Sheng, Xinxin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a210t-e1e2a79fc157eec2a16694d2200d1f4463168b13465fe2f107b49c7553c0ebc3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Materials and Interfaces</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Fan, Yawen</creatorcontrib><creatorcontrib>Wu, Jiongxin</creatorcontrib><creatorcontrib>Zhang, Li</creatorcontrib><creatorcontrib>Sheng, Xinxin</creatorcontrib><collection>CrossRef</collection><jtitle>Industrial & engineering chemistry research</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Fan, Yawen</au><au>Wu, Jiongxin</au><au>Zhang, Li</au><au>Sheng, Xinxin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Self-Oriented Functionalized MXene with Excellent Antioxidant Properties for Enhancing Anticorrosion Properties of Waterborne Epoxy Resin</atitle><jtitle>Industrial & engineering chemistry research</jtitle><addtitle>Ind. Eng. Chem. Res</addtitle><date>2024-06-19</date><risdate>2024</risdate><volume>63</volume><issue>24</issue><spage>10637</spage><epage>10650</epage><pages>10637-10650</pages><issn>0888-5885</issn><eissn>1520-5045</eissn><abstract>A MXene/poly(dimethyl diallyl ammonium chloride) (PDDA)/Fe3O4 (MPF) hybrid with exceptional oxidation resistance was synthesized via electrostatic self-assembly. Subsequently, a magnetic field was utilized to construct the parallel-aligned MPF within the waterborne epoxy coating (WEC). This parallel-aligned hybrid could significantly hinder the penetration of the corrosive ions. The electrochemical impedance spectroscopy (EIS) results revealed that the WEC containing parallel-aligned MPF (VMPF/WEC) exhibited the highest low-frequency impedance modulus (|Z 0.01 Hz|) among all coatings, which was 3 orders of magnitude higher than that of WEC in the initial stage of corrosion. After 42 days of the corrosion, the |Z 0.01 Hz| of VMPF/WEC surpassed that of WEC by more than 2 orders of magnitude, thereby indicating the exceptional long-term corrosion resistance of VMPF/WEC. This work proposed novel ideas for constructing high-performance anticorrosion WECs.</abstract><pub>American Chemical Society</pub><doi>10.1021/acs.iecr.4c01100</doi><tpages>14</tpages><orcidid>https://orcid.org/0000-0001-7695-0430</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0888-5885 |
| ispartof | Industrial & engineering chemistry research, 2024-06, Vol.63 (24), p.10637-10650 |
| issn | 0888-5885 1520-5045 |
| language | eng |
| recordid | cdi_crossref_primary_10_1021_acs_iecr_4c01100 |
| source | American Chemical Society Journals |
| subjects | Materials and Interfaces |
| title | Self-Oriented Functionalized MXene with Excellent Antioxidant Properties for Enhancing Anticorrosion Properties of Waterborne Epoxy Resin |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-02T00%3A18%3A52IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-acs_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Self-Oriented%20Functionalized%20MXene%20with%20Excellent%20Antioxidant%20Properties%20for%20Enhancing%20Anticorrosion%20Properties%20of%20Waterborne%20Epoxy%20Resin&rft.jtitle=Industrial%20&%20engineering%20chemistry%20research&rft.au=Fan,%20Yawen&rft.date=2024-06-19&rft.volume=63&rft.issue=24&rft.spage=10637&rft.epage=10650&rft.pages=10637-10650&rft.issn=0888-5885&rft.eissn=1520-5045&rft_id=info:doi/10.1021/acs.iecr.4c01100&rft_dat=%3Cacs_cross%3Ec254464385%3C/acs_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_id=info:pmid/&rfr_iscdi=true |