Review on Action Mechanism and Characterization of Natural/Artificial Solid Electrolyte Interphase of Lithium Battery: Latest Progress and Future Directions

At present, the basic structure and mechanism of solid electrolyte interface (SEI) have been studied based on different models. Although many researchers have observed the characteristics and properties of SEI through various characterization methods, it is still unable to explain its dynamic mechan...

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Veröffentlicht in:Energy & fuels 2023-01, Vol.37 (2), p.833-857
Hauptverfasser: Yuan, Hang, Zheng, Guoxu, Zhang, Daqing, Yang, Xu
Format: Artikel
Sprache:eng
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Zusammenfassung:At present, the basic structure and mechanism of solid electrolyte interface (SEI) have been studied based on different models. Although many researchers have observed the characteristics and properties of SEI through various characterization methods, it is still unable to explain its dynamic mechanism of action from the very small microscopic level. Among them, most researchers change the electrochemical performance of batteries by adding additives or material coating. Traditional research methods only state the performance of batteries from the appearance but lack detailed analysis of the electrochemical reaction of batteries during the research process. Based on the analysis of some models established by SEI, this study summarized the analysis of the research angle of SEI film through various characterization methods. The present traditional SEI and artificial SEI are introduced. Finally, the methods to improve the chemical performance of lithium battery and the challenges to solve the problems are summarized and prospected.
ISSN:0887-0624
1520-5029
DOI:10.1021/acs.energyfuels.2c02920