Solution-processed PEDOT:PSS:GO/Ag NWs composite electrode for flexible organic light-emitting diodes

[Display omitted] •The PEDOT:PSS:GO/Ag NWs flexible electrodes were prepared by two-steps solution method with the transmittance and sheet resistance of 88.7% and 17 Ω/sq, respectively.•The performance of OLEDs based on PEDOT:PSS:GO/Ag NWs was superior to that based on ITO.•The enhanced performance...

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Veröffentlicht in:Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy Molecular and biomolecular spectroscopy, 2021-03, Vol.248, p.119267, Article 119267
Hauptverfasser: Du, Hui, Guo, Yangyang, Cui, Dongyue, Li, Shuhong, Wang, Wenjun, Liu, Yunlong, Yao, Yicun, Zhao, Ling, Dong, Xiaochen
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Sprache:eng
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Zusammenfassung:[Display omitted] •The PEDOT:PSS:GO/Ag NWs flexible electrodes were prepared by two-steps solution method with the transmittance and sheet resistance of 88.7% and 17 Ω/sq, respectively.•The performance of OLEDs based on PEDOT:PSS:GO/Ag NWs was superior to that based on ITO.•The enhanced performance of flexible OLEDs mainly attributed to the great performance parameters of the composite electrode, the Far SPR effect and lower waveguide optical loss because of the introduction of Ag NWs in the electrode. Flexible organic light emitting diodes (OLEDs) have attracted considerable attention for the reason of light weight, high mechanical flexibility in display and lighting. The most widely used transparent anode indium tin oxide (ITO) is unsuitable for flexible OLEDs because of its easy cracking upon bending. In this paper, we proposed a simple two steps solution processing method to fabricate flexible PEDOT:PSS:GO/Ag NWs composite electrodes. The optimized PEDOT:PSS:GO/Ag NWs composite electrode exhibits an optical transmittance of 88.7% at a wavelength of 550 nm and a low sheet resistance of 17 Ω/sq, which arecomparable to that of ITO. With PEDOT:PSS:GO/Ag NWs composite electrodes, the turn on voltage, current density and maximum brightness of OLEDs based on composite electrode were 2.1 V, 6.2 cd/A and 22894 cd/m2, respectively, which were superior to that OLED based on ITO anode. The enhanced performance of OLEDs based on composite anode mainly attributed to the lower sheet resistance, smoother surface of the composite anode and the far surface plasma resonance (Far SPR) effect, a lower waveguide optical loss because of the introduction of Ag NWs in the electrode.
ISSN:1386-1425
1873-3557
DOI:10.1016/j.saa.2020.119267