N/S co-doped carbon nanosheets derived from sugarcane processing by-products for flexible solid-state supercapacitors
[Display omitted] •N/S co-doped carbon nanosheets derived from sugarcane processing by-products are synthesized.•Sulfonated potassium fulvic acid is used as both carbon source and heteroatom dopant.•The symmetric supercapacitor delivers a maximum energy and power density of 0.92 mW cm−2 and 184.5 μW...
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Veröffentlicht in: | Journal of electroanalytical chemistry (Lausanne, Switzerland) Switzerland), 2023-03, Vol.932, p.117217, Article 117217 |
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Format: | Artikel |
Sprache: | eng |
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•N/S co-doped carbon nanosheets derived from sugarcane processing by-products are synthesized.•Sulfonated potassium fulvic acid is used as both carbon source and heteroatom dopant.•The symmetric supercapacitor delivers a maximum energy and power density of 0.92 mW cm−2 and 184.5 μWh cm−2, respectively.
Developing sustainable carbon materials from biomass for supercapacitors is a promising solution to alleviate energy and environmental pressures. In this paper, novel N/S co-doped carbon nanosheets derived from sugarcane processing by-products are proposed. Flexible and binder-free electrodes based on carbon felt and sulfonated potassium fulvic acid were prepared by a simple impregnation-carbonization method. The maximum areal specific capacitance, power density and energy density of the symmetric supercapacitor are 409.9 mF cm−2 (1 mA cm−2), 0.92 mW cm−2 and 184.5 μWh cm−2, respectively. The operating voltage of the device increases to 1.8 V by using LiCl electrolyte. After 10,000 cycles, the capacitance remains 90 % of its initial value. Besides, the device possesses good flexibility, which can be bent at different angles and has a capacitance retention of 92.3 % after 5000 bending cycles. The supercapacitor is of great significance for the recovery of crop processing by-products to prepare flexible electronic devices. |
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ISSN: | 1572-6657 1873-2569 |
DOI: | 10.1016/j.jelechem.2023.117217 |