Porosity and permeability optimization of PEMFC cathode gas diffusion layer based on topology algorithm

The gas diffusion layer (GDL) is a crucial component in proton exchange membrane fuel cells (PEMFCs), significantly affecting mass transport and overall cell performance. Due to the pronounced pressure gradients and uneven mass transfer between the inlet and outlet of the serpentine flow field, this...

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Veröffentlicht in:International journal of electrochemical science 2024-11, Vol.19 (11), p.100803, Article 100803
Hauptverfasser: Zheng, Minggang, Liang, Han, Bu, Wenxie, Qu, Cheng, Hu, Xiaoxu, Zhang, Zhihu
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Sprache:eng
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Zusammenfassung:The gas diffusion layer (GDL) is a crucial component in proton exchange membrane fuel cells (PEMFCs), significantly affecting mass transport and overall cell performance. Due to the pronounced pressure gradients and uneven mass transfer between the inlet and outlet of the serpentine flow field, this study proposes the design of a GDL with a concentration gradient to optimize performance. Leveraging topological optimization algorithms, the research focuses on enhancing the mass transport properties and improving cell efficiency. The optimization process considers the pressure distribution, oxygen concentration, and water content within the serpentine flow field as boundary conditions. By optimizing the porosity and permeability of the GDL in different regions, the study aims to enhance the GDL's mass transport capabilities. Simulation results demonstrate that initializing the porosity at 1 provides superior optimization, significantly enhancing mass transfer and overall cell performance. Although increased permeability contributes to improved mass transport, its impact is less significant compared to porosity optimization. Therefore, GDL porosity is identified as the dominant factor in enhancing cell performance, while permeability adjustments play a secondary role.
ISSN:1452-3981
1452-3981
DOI:10.1016/j.ijoes.2024.100803