Polarization-Induced Two-Dimensional electron gas at BeO/ZnO interface

[Display omitted] •Beryllium oxide (BeO) films are grown on ZnO substrates via atomic layer deposition.•BeO films grown in a wurtzite structure along the c-axis induce a polarization discontinuity.•Polarization-induced two-dimensional electron gas (2DEG) occurs at a BeO/ZnO Interface.•Carrier concen...

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Veröffentlicht in:Applied surface science 2022-10, Vol.600, p.154103, Article 154103
Hauptverfasser: Jang, Yoonseo, Jung, Dohwan, Sultane, Prakash R., Bielawski, Christopher W., Oh, Jungwoo
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Sprache:eng
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Zusammenfassung:[Display omitted] •Beryllium oxide (BeO) films are grown on ZnO substrates via atomic layer deposition.•BeO films grown in a wurtzite structure along the c-axis induce a polarization discontinuity.•Polarization-induced two-dimensional electron gas (2DEG) occurs at a BeO/ZnO Interface.•Carrier concentration and mobility are 2.0 × 1014cm−2 and 22 cm2·V−1·s−1 at room temperature. Beryllium oxide (BeO) is a unique metal oxide with excellent thermal conductivity and dielectric strength. BeO tends to grow as wurtzite single crystals via atomic layer deposition, leading to the strong polarization of heterostructures with various substrates. We demonstrated the formation of a polarization-induced two-dimensional electron gas (2DEG) at a BeO/ZnO heterostructure interface. The polarity discontinuity induced by the c-axis-grown crystalline BeO film caused charges to accumulate on the ZnO substrate. The sheet carrier concentration and mobility of the BeO/ZnO heterostructure were 2.0 × 1014 cm−2 and 22 cm2·V−1·s−1 at room temperature, respectively, approximately 57 times and 11 times greater than those of bare ZnO, respectively. In addition, the carrier concentration was nearly constant over the temperature range of 150 K – 350 K. The 2DEG layers formed via ALD BeO films are possible channel materials for use in various electronic devices such as thin film transistors.
ISSN:0169-4332
1873-5584
DOI:10.1016/j.apsusc.2022.154103