Electron donor or acceptor behavior of a AuCl3 dopant manipulated by dip-pen nanolithography on a MoS2 thin-film transistor

[Display omitted] •AuCl3 doping in local area of the MoS2 was carried out by dip-pen nanolithography (DPN) with controlling the AuCl3 concentration.•Dependent on the AuCl3 concentration of the DPN process, AuCl3 dopant acts as electron acceptor or donor in the MoS2 thin-film transistor.•By utilizing...

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Veröffentlicht in:Applied surface science 2022-06, Vol.588, p.152846, Article 152846
Hauptverfasser: Park, Ki Hong, Jo, Jeong-Sik, Choi, Jinho, Kim, Min Jung, Chung, Kwun-Bum, Hong, Young Ki, Park, Dong Hyuk, Jang, Jae-Won
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Sprache:eng
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Zusammenfassung:[Display omitted] •AuCl3 doping in local area of the MoS2 was carried out by dip-pen nanolithography (DPN) with controlling the AuCl3 concentration.•Dependent on the AuCl3 concentration of the DPN process, AuCl3 dopant acts as electron acceptor or donor in the MoS2 thin-film transistor.•By utilizing this dopant concentration dependent type tunable local doping features through DPN, property of MoS2 application can be enhanced. Gold (III) chloride (AuCl3) is a well-known electron acceptor (p-type dopant). Here, the electron donor or acceptor behavior of a AuCl3 dopant on a molybdenum disulfide (MoS2) thin-film transistor (TFT) is demonstrated by line patterning a concentration-adjusted AuCl3 ink with dip-pen nanolithography (DPN). At a low ink concentration (clow) (
ISSN:0169-4332
1873-5584
DOI:10.1016/j.apsusc.2022.152846