Tunable luminescent color from green to blue on long afterglow materials using CsPbBr3 quantum dots

[Display omitted] •Prepared the color-tunable material CsPbBr3/SMS@SiO2 for the first time.•Improve the stability of CsPbBr3 and composite materials by wrapping SiO2.•The mechanism of perovskite quantum dots as light conversion materials. The single color of long afterglow luminescence materials is...

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Veröffentlicht in:Applied surface science 2021-12, Vol.568, p.150941, Article 150941
Hauptverfasser: Hai, Ou, Pei, Mengkang, Yang, Enlong, Ren, Qiang, Wu, Xiulan, Zhao, Yujing, Du, Liang
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Sprache:eng
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Zusammenfassung:[Display omitted] •Prepared the color-tunable material CsPbBr3/SMS@SiO2 for the first time.•Improve the stability of CsPbBr3 and composite materials by wrapping SiO2.•The mechanism of perovskite quantum dots as light conversion materials. The single color of long afterglow luminescence materials is one of the important factors restricting its development. Here, we uniformly disperse all-inorganic cesium lead halide (CsPbBr3) perovskite quantum dots (PeQDs) with strong stability on the surface of Sr2MgSi2O7:Eu2+,Dy3+ (SMS) to adjust the afterglow luminescence color. CsPbBr3 PeQDs has high quantum yield, and its excitation spectrum (around 400–500 nm) overlaps with the emission spectrum (around 465 nm) of SMS, so that the tunable afterglow emission from blue (around 465 nm) to green (around 525 nm) can be achieved by controlling the dosage of CsPbBr3 PeQDs, and its chromaticity coordinates can be from (0.1280, 0.1360) to (0.2010, 0, 7460). The quantum yield of the composite remains almost unchanged, and the luminescence intensity remains stable and does not decrease when the composite is irradiated by ultraviolet light for 2 h; When exposed to air, the luminescence property remained about 80 percent after 10 days. This study provides a research direction for the polychromatic adjustment of long afterglow luminescent materials.
ISSN:0169-4332
1873-5584
DOI:10.1016/j.apsusc.2021.150941