Peracetic acid-induced nanoengineering of Fe-based metallic glass ribbon in application of efficient drinking water treatment

This study presents a novel approach utilizing Fe-Si-B metallic glass-based advanced oxidation processes (AOPs) with peracetic acid (PAA) exposure to mitigate disinfection by-products (DBPs) formation in drinking water treatment. Under optimal conditions, it achieved a 98.21% removal of natural orga...

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Veröffentlicht in:Applied catalysis. B, Environmental Environmental, 2024-10, Vol.355, p.124161, Article 124161
Hauptverfasser: Li, Yujian, Liu, Yan, Zhan, Yangguang, Zhang, Yu, Zhao, Xingran, Yang, Mengting, Ruan, Wenqing, Zhang, Zhenxuan, Liang, Xiong, Ma, Jiang
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Sprache:eng
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Zusammenfassung:This study presents a novel approach utilizing Fe-Si-B metallic glass-based advanced oxidation processes (AOPs) with peracetic acid (PAA) exposure to mitigate disinfection by-products (DBPs) formation in drinking water treatment. Under optimal conditions, it achieved a 98.21% removal of natural organic matter (NOM) and an 80.64% reduction in DBPs formation. The efficacy is attributed to the galvanic cell effect induced by nanoflower structures on the ribbon surface, produced via PAA exposure, thereby enhancing degradation efficiency. High-valent iron Fe(IV) was identified as the primary reactive species, showing robust cycling efficiency under near-neutral conditions. Continuous flow experiments and toxicity assessments using luminescent bacteria further validated the method, demonstrating minimal metal leaching (
ISSN:0926-3373
1873-3883
DOI:10.1016/j.apcatb.2024.124161