Performance study and comparison between catalytic static mixer and packed bed in heterogeneous hydrogenation of vinyl acetate

Catalytic Static Mixers (CSMs) used in a continuous flow reactor for heterogeneous catalysis have been compared with packed bed reactor technology for the hydrogenation of vinyl acetate to ethyl acetate over 5 wt-% Pd/Al 2 O 3 catalyst. The CSM reactor showed lower pressure drop, better heat transfe...

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Veröffentlicht in:Journal of flow chemistry 2021-09, Vol.11 (3), p.515-523
Hauptverfasser: Zhu, Yutong, Bin Mohamad Sultan, Borhan, Nguyen, Xuan, Hornung, Christian
Format: Artikel
Sprache:eng
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Zusammenfassung:Catalytic Static Mixers (CSMs) used in a continuous flow reactor for heterogeneous catalysis have been compared with packed bed reactor technology for the hydrogenation of vinyl acetate to ethyl acetate over 5 wt-% Pd/Al 2 O 3 catalyst. The CSM reactor showed lower pressure drop, better heat transfer, and higher conversion and turnover frequency compared to a traditional packed bed reactor. A reaction performance study with varying CSM length has been performed and shows that the hydrogenation reactions are limited by the chemical reaction kinetics and not by the mass transfer.
ISSN:2062-249X
2063-0212
DOI:10.1007/s41981-021-00152-7