Synchrotron based conversion electron Mössbauer spectroscopy

Advanced conversion electron Mössbauer spectroscopy (CEMS) techniques using a synchrotron Mössbauer source (SMS) have been developed at BL11XU of SPring-8. The excellent beam properties of SMS γ-rays, such as fully recoilless, extremely high brilliance, a small beam size, and pure linear polarizatio...

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Veröffentlicht in:Hyperfine interactions 2024-11, Vol.245 (1), Article 347
Hauptverfasser: Mitsui, Takaya, Fujiwara, Kosuke, Sakai, Seiji, Li, Songtian, Okabayashi, Jun, Kobayashi, Yasuhiro, Seto, Makoto
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Sprache:eng
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Zusammenfassung:Advanced conversion electron Mössbauer spectroscopy (CEMS) techniques using a synchrotron Mössbauer source (SMS) have been developed at BL11XU of SPring-8. The excellent beam properties of SMS γ-rays, such as fully recoilless, extremely high brilliance, a small beam size, and pure linear polarization, facilitate sample measurements in special environments and micro-Mössbauer spectroscopy. This paper describes the development of instrumentation and demonstration for 57 Fe nuclei using the synchrotron-based CEMS, including in-situ CEMS of a magnetic thin film under cryogenic and ultra-high vacuum conditions, operando CEMS of a voltage-applied magnetic/dielectric thin film, and local region Mössbauer analysis of weathering steel using micro-focused SMS γ-rays.
ISSN:3005-0731
0304-3843
3005-0731
1572-9540
DOI:10.1007/s10751-024-02195-3