Elucidation of Metal Local Environments in Single‐Atom Catalysts Based on Carbon Nitrides (Small 33/2022)

Single‐Atom Catalysts In article number 2202080, Javier Pérez‐Ramírez, Sharon Mitchell, and co‐workers analyze the local environment of platinum in single‐atom catalysts based on poly(triazine imide) by atomic‐resolution imaging, various spectroscopies, and density functional theory. The experimenta...

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Veröffentlicht in:Small (Weinheim an der Bergstrasse, Germany) Germany), 2022-08, Vol.18 (33), p.n/a
Hauptverfasser: Büchele, Simon, Yakimov, Alexander, Collins, Sean M., Ruiz‐Ferrando, Andrea, Chen, Zupeng, Willinger, Elena, Kepaptsoglou, Demie M., Ramasse, Quentin M., Müller, Christoph R., Safonova, Olga V., López, Núria, Copéret, Christophe, Pérez‐Ramírez, Javier, Mitchell, Sharon
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Sprache:eng
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Zusammenfassung:Single‐Atom Catalysts In article number 2202080, Javier Pérez‐Ramírez, Sharon Mitchell, and co‐workers analyze the local environment of platinum in single‐atom catalysts based on poly(triazine imide) by atomic‐resolution imaging, various spectroscopies, and density functional theory. The experimental data corroborate theoretical predictions that metal atoms primarily localize in‐plane near the corners of the intrinsic scaffold cavities and expose the site diversity within the catalytic material.
ISSN:1613-6810
1613-6829
DOI:10.1002/smll.202270175