H 2 S Reactive Absorption from Off‐Gas in a Spray Column: Insights from Experiments and Modeling
H 2 S removal from an off‐gas stream was performed in a spray column by H 2 S reactive absorption into a NaOH solution. The individual and interactive effects of three independent operating variables on the percentage of absorbed H 2 S were investigated: the initial pH of the scrubbing solution, the...
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Veröffentlicht in: | Chemical engineering & technology 2015-12, Vol.38 (12), p.2137-2145 |
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Hauptverfasser: | , , |
Format: | Artikel |
Sprache: | eng |
Online-Zugang: | Volltext |
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Zusammenfassung: | H
2
S removal from an off‐gas stream was performed in a spray column by H
2
S reactive absorption into a NaOH solution. The individual and interactive effects of three independent operating variables on the percentage of absorbed H
2
S were investigated: the initial pH of the scrubbing solution, the initial scrubbing solution temperature, and the volumetric liquid‐to‐gas ratio. The optimum operating variables were determined by response surface methodology (RSM) attaining a percentage of absorbed H
2
S of 98.7 ± 0.2 %. Additionally, the process performance was modeled by an artificial neural network (ANN) to predict the percentage of absorbed H
2
S. The results showed that the experimental data agreed better with the ANN model than with the RSM results. |
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ISSN: | 0930-7516 1521-4125 |
DOI: | 10.1002/ceat.201500233 |