Spiral Spin Liquid State in the Corrugated Honeycomb Lattice of CaMn$_2$P$_2
CaMn$_2$P$_2$ exemplifies the realization of a frustrated $J_1$-$J_2$-$J_3$ Heisenberg model of a corrugated honeycomb magnetic lattice. Previous studies show that below the N\'eel temperature ($T_{\rm N}$), the system forms a cycloidal $6\times 6$ $ab$-plane magnetic unit cell that conforms wi...
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Zusammenfassung: | CaMn$_2$P$_2$ exemplifies the realization of a frustrated $J_1$-$J_2$-$J_3$
Heisenberg model of a corrugated honeycomb magnetic lattice. Previous studies
show that below the N\'eel temperature ($T_{\rm N}$), the system forms a
cycloidal $6\times 6$ $ab$-plane magnetic unit cell that conforms with various
magnetic space groups. Here, we present single-crystal neutron-diffraction
studies across expansive reciprocal-space volumes, confirming the cycloidal
magnetic structure while uncovering further distinctive features. We find
evidence for three magnetic domains, the analysis of which narrows the possible
magnetic model structures. At $T_{\rm N}$, the insulator exhibits a sharp phase
transition, above which the spin structure transforms into a spiral spin liquid
state, evident via a continuous ring of scattering with degenerate wavevectors
corresponding to a collection of short-range spiral spin configurations. These
degenerate states emerge as thermal fluctuations effectively reduce the $J_3$
interaction. The integration of experimental, theoretical, and real-space
simulation results reveals the intricate balance of exchange interactions
($J_1$-$J_2$-$J_3$) that stabilizes the ground-state magnetic structure and
drives the emergence of a sought-after $U$(1)-symmetric spiral spin-liquid
state with easy-plane anisotropy above the transition temperature. |
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DOI: | 10.48550/arxiv.2501.02122 |