YbNi$_4$Mg: Superheavy fermion with enhanced Wilson ratio and magnetocaloric effect
A comprehensive study of the low-temperature properties of YbNi$_4$Mg has revealed evidence of a superheavy-fermion state, characterized by a large electronic specific-heat coefficient $\gamma_0$ $\approx$ 5.65 J mol$^{-1}$ K$^{-2}$ and an elevated Wilson ratio $R_W$ = 32.1. No magnetic ordering was...
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Zusammenfassung: | A comprehensive study of the low-temperature properties of YbNi$_4$Mg has
revealed evidence of a superheavy-fermion state, characterized by a large
electronic specific-heat coefficient $\gamma_0$ $\approx$ 5.65 J mol$^{-1}$
K$^{-2}$ and an elevated Wilson ratio $R_W$ = 32.1. No magnetic ordering was
observed down to 70 mK; however, a broad maximum appears in the specific heat
at $T^*$ = 0.3 K, along with a shoulder in the derivative of susceptibility
d$\chi$/d$T$ and resistivity d$\rho$/d$T$. These features indicate a
cooperative yet short-ranged magnetism entwined with the superheavy Fermi
liquid. The large Wilson ratio, which is also detected in other
superheavy-fermion compounds lacking long-range order, might be a signature of
residual spin fluctuations. Applying a weak magnetic field of $\sim$0.1 T
induces a metamagnetic-like crossover, as demonstrated by the quasi-adiabatic
demagnetization measurements showing a broad minimum in the temperature-field
trace. Here, an enhanced magnetocaloric cooling effect stemming from the
field-sensitive superheavy-fermion state is observed, rivaling that of the
well-established insulating magnetic coolants like the rare-earth garnet
Gd$_3$Ga$_5$O$_{12}$. |
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DOI: | 10.48550/arxiv.2412.08043 |