Polarized Superradiance from CsPbBr3 Quantum Dot Superlattice with Controlled Inter-dot Electronic Coupling

Cooperative emission of photons from an ensemble of quantum dots (QDs) as superradiance can arise from the electronically coupled QDs with a coherent emitting excited state. This contrasts with superfluorescence (Dicke superradiance), where the cooperative photon emission occurs via a spontaneous bu...

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Hauptverfasser: Luo, Lanyin, Tang, Xueting, Park, Junhee, Wang, Chih-Wei, Park, Mansoo, Khurana, Mohit, Singh, Ashutosh, Cheon, Jinwoo, Belyanin, Alexey, Sokolov, Alexei V, Son, Dong Hee
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Sprache:eng
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Zusammenfassung:Cooperative emission of photons from an ensemble of quantum dots (QDs) as superradiance can arise from the electronically coupled QDs with a coherent emitting excited state. This contrasts with superfluorescence (Dicke superradiance), where the cooperative photon emission occurs via a spontaneous buildup of coherence in an ensemble of incoherently excited QDs via their coupling to a common radiation mode. While superfluorescence has been observed in perovskite QD systems, reports of superradiance from the electronically coupled ensemble of perovskite QDs are rare. Here, we demonstrate the generation of polarized superradiance with a very narrow linewidth (
DOI:10.48550/arxiv.2411.09051