Charge Density Fluctuations with Enhanced Superconductivity at the Proposed Nematic Quantum Critical Point
A quantum critical point (QCP) represents a continuous phase transition at absolute zero. At the QCP of an unconventional superconductor, enhanced superconducting transition temperature and magnetic fluctuations strength are often observed together, indicating magnetism-mediated superconductivity. T...
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Zusammenfassung: | A quantum critical point (QCP) represents a continuous phase transition at
absolute zero. At the QCP of an unconventional superconductor, enhanced
superconducting transition temperature and magnetic fluctuations strength are
often observed together, indicating magnetism-mediated superconductivity. This
raises the question of whether quantum fluctuations in other degrees of
freedom, such as charge, could similarly boost superconductivity. However,
because charge is frequently intertwined with magnetism, isolating and
understanding its specific role in Cooper pair formation poses a significant
challenge. Here, we report persistent charge density fluctuations (CDF) down to
15 K in the non-magnetic superconductor Sr$_{0.77}$Ba$_{0.23}$Ni$_{2}$As$_{2}$,
which lies near a proposed nematic QCP associated with a six-fold enhancement
of superconductivity. Our results show that the quasi-elastic CDF does not
condense into resolution-limited Bragg peaks and displays non-saturated
strength. The CDF completely softens at 25 K, with its critical behavior
described by the same mathematical framework as the antiferromagnetic Fermi
liquid model, yielding a fitted Curie-Weiss temperature of $\theta \approx 0$
K. Additionally, we find that the nematic fluctuations are not lattice-driven,
as evidenced by the absence of softening in nematic-coupled in-plane transverse
acoustic phonons. Our discovery positions Sr$_{x}$Ba$_{1-x}$Ni$_{2}$As$_{2}$ as
a promising candidate for charge-fluctuation-driven nematicity and
superconductivity. |
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DOI: | 10.48550/arxiv.2410.03956 |