Realization of Z$_2$ topological photonic insulators made from multilayer transition metal dichalcogenides
Monolayers of semiconducting transition metal dichalcogenides (TMDs) have long attracted interest for their intriguing optical and electronic properties. Recently TMDs in their quasi-bulk form have started to show considerable promise for nanophotonics thanks to their high refractive indices, large...
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Zusammenfassung: | Monolayers of semiconducting transition metal dichalcogenides (TMDs) have
long attracted interest for their intriguing optical and electronic properties.
Recently TMDs in their quasi-bulk form have started to show considerable
promise for nanophotonics thanks to their high refractive indices, large
optical anisotropy, wide transparency windows reaching to the visible, and
robust room temperature excitons promising for nonlinear optics. Adherence of
TMD layers to any substrate via van der Waals forces is a further key enabler
for nanofabrication of sophisticated photonic structures requiring
heterointegration. Here, we capitalize on these attractive properties and
realize topological spin-Hall photonic lattices made of arrays of triangular
nanoholes in 50 to 100 nm thick WS$_2$ flakes exfoliated on SiO$_2$/Si
substrates. High quality structures are achieved taking advantage of
anisotropic dry etching dictated by the crystal axes of WS$_2$. Reflectance
measurements at room temperature show a photonic gap opening in the
near-infrared in trivial and topological phases. Unidirectional propagation
along the domain interface is demonstrated in real space via circularly
polarized laser excitation in samples with both zigzag and armchair domain
boundaries. Finite-difference time-domain simulations are used to interpret
optical spectroscopy results. Our work opens the way for future sophisticated
nanophotonic devices based on the layered (van der Waals) materials platform. |
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DOI: | 10.48550/arxiv.2407.05908 |