Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er$_2$Be$_2$SiO$_7
Polycrystalline and single crystal samples of the insulating Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a solid-state reaction and the floating zone method respectively. The crystal structure, Er single ion anisotropy, zero-field magnetic ground state, and magnetic phase di...
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creator | Brassington, A Ma, 1 Q Sala, G Kolesnikov, A. I Taddei, K. M Wu, Y Choi, E. S Wang, H Xie, W Ma, J Zhou, H. D Aczel, A. A |
description | Polycrystalline and single crystal samples of the insulating
Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a
solid-state reaction and the floating zone method respectively. The crystal
structure, Er single ion anisotropy, zero-field magnetic ground state, and
magnetic phase diagrams along high-symmetry crystallographic directions were
investigated by bulk measurement techniques, x-ray and neutron diffraction, and
neutron spectroscopy. We establish that Er$_2$Be$_2$SiO$_7$ crystallizes in a
tetragonal space group with planes of orthogonal Er dimers and a strong
preference for the Er moments to lie in the local plane perpendicular to each
dimer bond. We also find that this system has a non-collinear ordered ground
state in zero field with a transition temperature of 0.841 K consisting of
antiferromagnetic dimers and in-plane moments. Finally, we mapped out the $H-T$
phase diagrams for Er$_2$Be$_2$SiO$_7$ along the directions $H \parallel$
[001], [100], and [110]. While an increasing in-plane field simply induces a
phase transition to a field-polarized phase, we identify three metamagnetic
transitions before the field-polarized phase is established in the $H
\parallel$ [001] case. This complex behavior establishes insulating
Er$_2$Be$_2$SiO$_7$ and other isostructural family members as promising
candidates for uncovering exotic magnetic properties and phenomena that can be
readily compared to theoretical predictions of the exactly soluble
Shastry-Sutherland model. |
doi_str_mv | 10.48550/arxiv.2405.08230 |
format | Article |
fullrecord | <record><control><sourceid>arxiv_GOX</sourceid><recordid>TN_cdi_arxiv_primary_2405_08230</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2405_08230</sourcerecordid><originalsourceid>FETCH-LOGICAL-a670-96590c4862d54a237bf59731eedf9a9b89362ea1c81b5e6322f7a2c8e4e28b453</originalsourceid><addsrcrecordid>eNotjztPwzAUhb0woMIPYKqHrA6OX7FHqMpDKipSOpTJukmuqaU-gpMi-u9pA8s50pG-I32E3BU8V1Zrfg_pJ37nQnGdcyskvybvb_C5xyE2tEuHDtMQsaeHQIcN0q8j9JGtP2i1gX5IJ1Ydz3Pawr6luxGj85R5kT3iJau4zHx5Q64CbHu8_e8JWT3NV7MXtlg-v84eFgxMyZkz2vFGWSNarUDIsg7albJAbIMDV1snjUAoGlvUGo0UIpQgGosKha2VlhMy_bsdlXyX4g7SyV_U_KgmfwEoQ0dx</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype></control><display><type>article</type><title>Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er$_2$Be$_2$SiO$_7</title><source>arXiv.org</source><creator>Brassington, A ; Ma, 1 Q ; Sala, G ; Kolesnikov, A. I ; Taddei, K. M ; Wu, Y ; Choi, E. S ; Wang, H ; Xie, W ; Ma, J ; Zhou, H. D ; Aczel, A. A</creator><creatorcontrib>Brassington, A ; Ma, 1 Q ; Sala, G ; Kolesnikov, A. I ; Taddei, K. M ; Wu, Y ; Choi, E. S ; Wang, H ; Xie, W ; Ma, J ; Zhou, H. D ; Aczel, A. A</creatorcontrib><description>Polycrystalline and single crystal samples of the insulating
Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a
solid-state reaction and the floating zone method respectively. The crystal
structure, Er single ion anisotropy, zero-field magnetic ground state, and
magnetic phase diagrams along high-symmetry crystallographic directions were
investigated by bulk measurement techniques, x-ray and neutron diffraction, and
neutron spectroscopy. We establish that Er$_2$Be$_2$SiO$_7$ crystallizes in a
tetragonal space group with planes of orthogonal Er dimers and a strong
preference for the Er moments to lie in the local plane perpendicular to each
dimer bond. We also find that this system has a non-collinear ordered ground
state in zero field with a transition temperature of 0.841 K consisting of
antiferromagnetic dimers and in-plane moments. Finally, we mapped out the $H-T$
phase diagrams for Er$_2$Be$_2$SiO$_7$ along the directions $H \parallel$
[001], [100], and [110]. While an increasing in-plane field simply induces a
phase transition to a field-polarized phase, we identify three metamagnetic
transitions before the field-polarized phase is established in the $H
\parallel$ [001] case. This complex behavior establishes insulating
Er$_2$Be$_2$SiO$_7$ and other isostructural family members as promising
candidates for uncovering exotic magnetic properties and phenomena that can be
readily compared to theoretical predictions of the exactly soluble
Shastry-Sutherland model.</description><identifier>DOI: 10.48550/arxiv.2405.08230</identifier><language>eng</language><subject>Physics - Other Condensed Matter ; Physics - Strongly Correlated Electrons</subject><creationdate>2024-05</creationdate><rights>http://creativecommons.org/licenses/by/4.0</rights><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>228,230,776,881</link.rule.ids><linktorsrc>$$Uhttps://arxiv.org/abs/2405.08230$$EView_record_in_Cornell_University$$FView_record_in_$$GCornell_University$$Hfree_for_read</linktorsrc><backlink>$$Uhttps://doi.org/10.48550/arXiv.2405.08230$$DView paper in arXiv$$Hfree_for_read</backlink></links><search><creatorcontrib>Brassington, A</creatorcontrib><creatorcontrib>Ma, 1 Q</creatorcontrib><creatorcontrib>Sala, G</creatorcontrib><creatorcontrib>Kolesnikov, A. I</creatorcontrib><creatorcontrib>Taddei, K. M</creatorcontrib><creatorcontrib>Wu, Y</creatorcontrib><creatorcontrib>Choi, E. S</creatorcontrib><creatorcontrib>Wang, H</creatorcontrib><creatorcontrib>Xie, W</creatorcontrib><creatorcontrib>Ma, J</creatorcontrib><creatorcontrib>Zhou, H. D</creatorcontrib><creatorcontrib>Aczel, A. A</creatorcontrib><title>Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er$_2$Be$_2$SiO$_7</title><description>Polycrystalline and single crystal samples of the insulating
Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a
solid-state reaction and the floating zone method respectively. The crystal
structure, Er single ion anisotropy, zero-field magnetic ground state, and
magnetic phase diagrams along high-symmetry crystallographic directions were
investigated by bulk measurement techniques, x-ray and neutron diffraction, and
neutron spectroscopy. We establish that Er$_2$Be$_2$SiO$_7$ crystallizes in a
tetragonal space group with planes of orthogonal Er dimers and a strong
preference for the Er moments to lie in the local plane perpendicular to each
dimer bond. We also find that this system has a non-collinear ordered ground
state in zero field with a transition temperature of 0.841 K consisting of
antiferromagnetic dimers and in-plane moments. Finally, we mapped out the $H-T$
phase diagrams for Er$_2$Be$_2$SiO$_7$ along the directions $H \parallel$
[001], [100], and [110]. While an increasing in-plane field simply induces a
phase transition to a field-polarized phase, we identify three metamagnetic
transitions before the field-polarized phase is established in the $H
\parallel$ [001] case. This complex behavior establishes insulating
Er$_2$Be$_2$SiO$_7$ and other isostructural family members as promising
candidates for uncovering exotic magnetic properties and phenomena that can be
readily compared to theoretical predictions of the exactly soluble
Shastry-Sutherland model.</description><subject>Physics - Other Condensed Matter</subject><subject>Physics - Strongly Correlated Electrons</subject><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><sourceid>GOX</sourceid><recordid>eNotjztPwzAUhb0woMIPYKqHrA6OX7FHqMpDKipSOpTJukmuqaU-gpMi-u9pA8s50pG-I32E3BU8V1Zrfg_pJ37nQnGdcyskvybvb_C5xyE2tEuHDtMQsaeHQIcN0q8j9JGtP2i1gX5IJ1Ydz3Pawr6luxGj85R5kT3iJau4zHx5Q64CbHu8_e8JWT3NV7MXtlg-v84eFgxMyZkz2vFGWSNarUDIsg7albJAbIMDV1snjUAoGlvUGo0UIpQgGosKha2VlhMy_bsdlXyX4g7SyV_U_KgmfwEoQ0dx</recordid><startdate>20240513</startdate><enddate>20240513</enddate><creator>Brassington, A</creator><creator>Ma, 1 Q</creator><creator>Sala, G</creator><creator>Kolesnikov, A. I</creator><creator>Taddei, K. M</creator><creator>Wu, Y</creator><creator>Choi, E. S</creator><creator>Wang, H</creator><creator>Xie, W</creator><creator>Ma, J</creator><creator>Zhou, H. D</creator><creator>Aczel, A. A</creator><scope>GOX</scope></search><sort><creationdate>20240513</creationdate><title>Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er$_2$Be$_2$SiO$_7</title><author>Brassington, A ; Ma, 1 Q ; Sala, G ; Kolesnikov, A. I ; Taddei, K. M ; Wu, Y ; Choi, E. S ; Wang, H ; Xie, W ; Ma, J ; Zhou, H. D ; Aczel, A. A</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a670-96590c4862d54a237bf59731eedf9a9b89362ea1c81b5e6322f7a2c8e4e28b453</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Physics - Other Condensed Matter</topic><topic>Physics - Strongly Correlated Electrons</topic><toplevel>online_resources</toplevel><creatorcontrib>Brassington, A</creatorcontrib><creatorcontrib>Ma, 1 Q</creatorcontrib><creatorcontrib>Sala, G</creatorcontrib><creatorcontrib>Kolesnikov, A. I</creatorcontrib><creatorcontrib>Taddei, K. M</creatorcontrib><creatorcontrib>Wu, Y</creatorcontrib><creatorcontrib>Choi, E. S</creatorcontrib><creatorcontrib>Wang, H</creatorcontrib><creatorcontrib>Xie, W</creatorcontrib><creatorcontrib>Ma, J</creatorcontrib><creatorcontrib>Zhou, H. D</creatorcontrib><creatorcontrib>Aczel, A. A</creatorcontrib><collection>arXiv.org</collection></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext_linktorsrc</fulltext></delivery><addata><au>Brassington, A</au><au>Ma, 1 Q</au><au>Sala, G</au><au>Kolesnikov, A. I</au><au>Taddei, K. M</au><au>Wu, Y</au><au>Choi, E. S</au><au>Wang, H</au><au>Xie, W</au><au>Ma, J</au><au>Zhou, H. D</au><au>Aczel, A. A</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er$_2$Be$_2$SiO$_7</atitle><date>2024-05-13</date><risdate>2024</risdate><abstract>Polycrystalline and single crystal samples of the insulating
Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a
solid-state reaction and the floating zone method respectively. The crystal
structure, Er single ion anisotropy, zero-field magnetic ground state, and
magnetic phase diagrams along high-symmetry crystallographic directions were
investigated by bulk measurement techniques, x-ray and neutron diffraction, and
neutron spectroscopy. We establish that Er$_2$Be$_2$SiO$_7$ crystallizes in a
tetragonal space group with planes of orthogonal Er dimers and a strong
preference for the Er moments to lie in the local plane perpendicular to each
dimer bond. We also find that this system has a non-collinear ordered ground
state in zero field with a transition temperature of 0.841 K consisting of
antiferromagnetic dimers and in-plane moments. Finally, we mapped out the $H-T$
phase diagrams for Er$_2$Be$_2$SiO$_7$ along the directions $H \parallel$
[001], [100], and [110]. While an increasing in-plane field simply induces a
phase transition to a field-polarized phase, we identify three metamagnetic
transitions before the field-polarized phase is established in the $H
\parallel$ [001] case. This complex behavior establishes insulating
Er$_2$Be$_2$SiO$_7$ and other isostructural family members as promising
candidates for uncovering exotic magnetic properties and phenomena that can be
readily compared to theoretical predictions of the exactly soluble
Shastry-Sutherland model.</abstract><doi>10.48550/arxiv.2405.08230</doi><oa>free_for_read</oa></addata></record> |
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subjects | Physics - Other Condensed Matter Physics - Strongly Correlated Electrons |
title | Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er$_2$Be$_2$SiO$_7 |
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