Magnetic properties of the quasi-XY Shastry-Sutherland magnet Er$_2$Be$_2$SiO$_7
Polycrystalline and single crystal samples of the insulating Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a solid-state reaction and the floating zone method respectively. The crystal structure, Er single ion anisotropy, zero-field magnetic ground state, and magnetic phase di...
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Zusammenfassung: | Polycrystalline and single crystal samples of the insulating
Shastry-Sutherland compound Er$_2$Be$_2$SiO$_7$ were synthesized via a
solid-state reaction and the floating zone method respectively. The crystal
structure, Er single ion anisotropy, zero-field magnetic ground state, and
magnetic phase diagrams along high-symmetry crystallographic directions were
investigated by bulk measurement techniques, x-ray and neutron diffraction, and
neutron spectroscopy. We establish that Er$_2$Be$_2$SiO$_7$ crystallizes in a
tetragonal space group with planes of orthogonal Er dimers and a strong
preference for the Er moments to lie in the local plane perpendicular to each
dimer bond. We also find that this system has a non-collinear ordered ground
state in zero field with a transition temperature of 0.841 K consisting of
antiferromagnetic dimers and in-plane moments. Finally, we mapped out the $H-T$
phase diagrams for Er$_2$Be$_2$SiO$_7$ along the directions $H \parallel$
[001], [100], and [110]. While an increasing in-plane field simply induces a
phase transition to a field-polarized phase, we identify three metamagnetic
transitions before the field-polarized phase is established in the $H
\parallel$ [001] case. This complex behavior establishes insulating
Er$_2$Be$_2$SiO$_7$ and other isostructural family members as promising
candidates for uncovering exotic magnetic properties and phenomena that can be
readily compared to theoretical predictions of the exactly soluble
Shastry-Sutherland model. |
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DOI: | 10.48550/arxiv.2405.08230 |