Using magnetic dynamics to measure the spin gap in a candidate Kitaev material

npj Quantum Materials 10, 15 (2025) Materials potentially hosting Kitaev spin-liquid states are considered crucial for realizing topological quantum computing. However, the intricate nature of spin interactions within these materials complicates the precise measurement of low-energy spin excitations...

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Hauptverfasser: Jiang, Xinyi, Qiu, Qingzheng, Peng, Cheng, Jang, Hoyoung, Chen, Wenjie, Jin, Xianghong, Yue, Li, Lee, Byungjune, Park, Sang-Youn, Kim, Minseok, Kim, Hyeong-Do, Cai, Xinqiang, Li, Qizhi, Dong, Tao, Wang, Nanlin, Turner, Joshua J, Li, Yuan, Wang, Yao, Peng, Yingying
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Sprache:eng
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Zusammenfassung:npj Quantum Materials 10, 15 (2025) Materials potentially hosting Kitaev spin-liquid states are considered crucial for realizing topological quantum computing. However, the intricate nature of spin interactions within these materials complicates the precise measurement of low-energy spin excitations indicative of fractionalized excitations. Using Na$_{2}$Co$_2$TeO$_{6}$ as an example, we study these low-energy spin excitations using the time-resolved resonant elastic x-ray scattering (tr-REXS). Our observations unveil remarkably slow spin dynamics at the magnetic peak, whose recovery timescale is several nanoseconds. This timescale aligns with the extrapolated spin gap of $\sim$ 1 $\mu$eV, obtained by density matrix renormalization group (DMRG) simulations in the thermodynamic limit. The consistency demonstrates the efficacy of tr-REXS in discerning low-energy spin gaps inaccessible to conventional spectroscopic techniques.
DOI:10.48550/arxiv.2405.03212