Ultrafast Band Structure Dynamics in Bulk 1$T$-VSe$_2
Complex materials encompassing different phases of matter can display new photoinduced metastable states differing from those attainable under equilibrium conditions. These states can be realized when energy is injected in the material following a non-equilibrium pathway, unbalancing the unperturbed...
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Zusammenfassung: | Complex materials encompassing different phases of matter can display new
photoinduced metastable states differing from those attainable under
equilibrium conditions. These states can be realized when energy is injected in
the material following a non-equilibrium pathway, unbalancing the unperturbed
energy landscape of the material. Guided by the fact that photoemission
experiments allow for detailed insights in the electronic band structure of
ordered systems, here we study bulk 1T-VSe$_2$ in its metallic and
charge-density-wave phase by time- and angle-resolved photoelectron
spectroscopy. After near-infrared optical excitation, the system shows a net
increase of the density of states in the energy range of the valence bands, in
the vicinity of the Fermi level, lasting for several picoseconds. We discuss
possible origins as band shifts or correlation effects on the basis of a band
structure analysis. Our results uncover the possibility of altering the
electronic band structure of bulk 1T-VSe$_2$ for low excitation fluences,
contributing to the understanding of light-induced electronic states. |
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DOI: | 10.48550/arxiv.2403.03805 |